Machine learning in scanning transmission electron microscopy

SV Kalinin, C Ophus, PM Voyles, R Erni… - Nature Reviews …, 2022 - nature.com
Scanning transmission electron microscopy (STEM) has emerged as a uniquely powerful
tool for structural and functional imaging of materials on the atomic level. Driven by …

Electron microscopy studies of soft nanomaterials

Z Lyu, L Yao, W Chen, FC Kalutantirige… - Chemical …, 2023 - ACS Publications
This review highlights recent efforts on applying electron microscopy (EM) to soft (including
biological) nanomaterials. We will show how developments of both the hardware and …

Single-defect phonons imaged by electron microscopy

X Yan, C Liu, CA Gadre, L Gu, T Aoki, TC Lovejoy… - Nature, 2021 - nature.com
Crystal defects affect the thermal and heat-transport properties of materials by scattering
phonons and modifying phonon spectra,,,,,,–. To appreciate how imperfections in solids …

Nanoscale imaging of phonon dynamics by electron microscopy

CA Gadre, X Yan, Q Song, J Li, L Gu, H Huyan, T Aoki… - Nature, 2022 - nature.com
Spatially resolved vibrational map** of nanostructures is indispensable to the
development and understanding of thermal nanodevices, modulation of thermal transport …

Single-atom vibrational spectroscopy in the scanning transmission electron microscope

FS Hage, G Radtke, DM Kepaptsoglou, M Lazzeri… - Science, 2020 - science.org
Single-atom impurities and other atomic-scale defects can notably alter the local vibrational
responses of solids and, ultimately, their macroscopic properties. Using high-resolution …

Optical excitations with electron beams: Challenges and opportunities

FJ Garcia de Abajo, V Di Giulio - ACS photonics, 2021 - ACS Publications
Free electron beams such as those employed in electron microscopes have evolved into
powerful tools to investigate photonic nanostructures with an unrivaled combination of …

Direct observation of highly confined phonon polaritons in suspended monolayer hexagonal boron nitride

N Li, X Guo, X Yang, R Qi, T Qiao, Y Li, R Shi, Y Li… - Nature Materials, 2021 - nature.com
Phonon polaritons enable light confinement at deep subwavelength scales, with potential
technological applications, such as subdiffraction imaging, sensing and engineering of …

Single-atom vibrational spectroscopy with chemical-bonding sensitivity

M Xu, DL Bao, A Li, M Gao, D Meng, A Li, S Du, G Su… - Nature Materials, 2023 - nature.com
Correlation of lattice vibrational properties with local atomic configurations in materials is
essential for elucidating functionalities that involve phonon transport in solids. Recent …

Spatiotemporal imaging of 2D polariton wave packet dynamics using free electrons

Y Kurman, R Dahan, HH Sheinfux, K Wang, M Yannai… - Science, 2021 - science.org
Coherent optical excitations in two-dimensional (2D) materials, 2D polaritons, can generate
a plethora of optical phenomena that arise from the extraordinary dispersion relations that …

Measuring phonon dispersion at an interface

R Qi, R Shi, Y Li, Y Sun, M Wu, N Li, J Du, K Liu… - Nature, 2021 - nature.com
The breakdown of translational symmetry at heterointerfaces leads to the emergence of new
phonon modes localized at the interface. These modes have an essential role in thermal …