Mechanism of charge transport in lithium thiophosphate

L Gigli, D Tisi, F Grasselli, M Ceriotti - Chemistry of Materials, 2024 - ACS Publications
Lithium ortho-thiophosphate (Li3PS4) has emerged as a promising candidate for solid-state
electrolyte batteries, thanks to its highly conductive phases, cheap components, and large …

Viscosity in water from first-principles and deep-neural-network simulations

C Malosso, L Zhang, R Car, S Baroni… - npj Computational …, 2022 - nature.com
We report on an extensive study of the viscosity of liquid water at near-ambient conditions,
performed within the Green-Kubo theory of linear response and equilibrium ab initio …

Heat transport in liquid water from first-principles and deep neural network simulations

D Tisi, L Zhang, R Bertossa, H Wang, R Car, S Baroni - Physical Review B, 2021 - APS
We compute the thermal conductivity of water within linear response theory from equilibrium
molecular dynamics simulations, by adopting two different approaches. In one, the potential …

Tuning the through-plane lattice thermal conductivity in van der Waals structures through rotational (dis) ordering

F Eriksson, E Fransson, C Linderälv, Z Fan, P Erhart - ACS nano, 2023 - ACS Publications
It has recently been demonstrated that MoS2 with irregular interlayer rotations can achieve
an extreme anisotropy in the lattice thermal conductivity (LTC), which is, for example, of …

Temperature- and vacancy-concentration-dependence of heat transport in Li3ClO from multi-method numerical simulations

P Pegolo, S Baroni, F Grasselli - npj Computational Materials, 2022 - nature.com
Despite governing heat management in any realistic device, the microscopic mechanisms of
heat transport in all-solid-state electrolytes are poorly known: existing calculations, all based …

[HTML][HTML] Investigating finite-size effects in molecular dynamics simulations of ion diffusion, heat transport, and thermal motion in superionic materials

F Grasselli - The Journal of Chemical Physics, 2022 - pubs.aip.org
The effects of the finite size of the simulation box in equilibrium molecular dynamics
simulations are investigated for prototypical superionic conductors of different types, namely …

Thermal transport of glasses via machine learning driven simulations

P Pegolo, F Grasselli - Frontiers in Materials, 2024 - frontiersin.org
Accessing the thermal transport properties of glasses is a major issue for the design of
production strategies of glass industry, as well as for the plethora of applications and …

Hydrodynamic finite-size scaling of the thermal conductivity in glasses

A Fiorentino, P Pegolo, S Baroni - npj Computational Materials, 2023 - nature.com
In the past few years, the theory of thermal transport in amorphous solids has been
substantially extended beyond the Allen-Feldman model. The resulting formulation, based …

Thermal transport of LiPS solid electrolytes with ab initio accuracy

D Tisi, F Grasselli, L Gigli, M Ceriotti - arxiv preprint arxiv:2401.12936, 2024 - arxiv.org
The vast amount of computational studies on electrical conduction in solid state electrolytes
is not mirrored by comparable efforts addressing thermal conduction, which has been …

Molecular simulations: past, present, and future (a Topical Issue in EPJB)

G Ciccotti, C Dellago, M Ferrario… - The European Physical …, 2022 - Springer
Molecular simulation (MS) could be concisely described as computational statistical
mechanics [1], ie, numerical methods combined with computer power to address physico …