[FeFe]-Hydrogenases: maturation and reactivity of enzymatic systems and overview of biomimetic models

JT Kleinhaus, F Wittkamp, S Yadav… - Chemical Society …, 2021 - pubs.rsc.org
While hydrogen plays an ever-increasing role in modern society, nature has utilized
hydrogen since a very long time as an energy carrier and storage molecule. Among the …

Structural and functional analogues of the active sites of the [Fe]-,[NiFe]-, and [FeFe]-hydrogenases

C Tard, CJ Pickett - Chemical reviews, 2009 - ACS Publications
This article sets out to review the chemistry relating to the synthesis of structural and
functional analogues of the three classes of hydrogenases. This chemistry has grown …

Earth-abundant hydrogen evolution electrocatalysts

JR McKone, SC Marinescu, BS Brunschwig… - Chemical …, 2014 - pubs.rsc.org
Splitting water to hydrogen and oxygen is a promising approach for storing energy from
intermittent renewables, such as solar power. Efficient, scalable solar-driven electrolysis …

Production of hydrogen by electrocatalysis: making the H–H bond by combining protons and hydrides

RM Bullock, AM Appel, ML Helm - Chemical Communications, 2014 - pubs.rsc.org
Generation of hydrogen by reduction of two protons by two electrons can be catalysed by
molecular electrocatalysts. Determination of the thermodynamic driving force for elimination …

Some general principles for designing electrocatalysts with hydrogenase activity

V Artero, M Fontecave - Coordination chemistry reviews, 2005 - Elsevier
Hydrogenases are enzymes that catalyze the reversible interconversion between hydrogen
and protons with remarkable efficiency. On the other hand, the design of synthetic …

Rapid Water Reduction to H2 Catalyzed by a Cobalt Bis(iminopyridine) Complex

BD Stubbert, JC Peters, HB Gray - Journal of the American …, 2011 - ACS Publications
A cobalt bis (iminopyridine) complex is a highly active electrocatalyst for water reduction,
with an estimated apparent second order rate constant k app≤ 107 M–1s–1 over a range of …

Electron and proton transfers at diiron dithiolate sites relevant to the catalysis of proton reduction by the [FeFe]-hydrogenases

JF Capon, F Gloaguen, FY Pétillon… - Coordination Chemistry …, 2009 - Elsevier
This review focuses on electron and proton transfers involving hexacarbonyl and substituted
{2Fe2S} complexes inspired from the active site of the [FeFe]-hydrogenases ([FeFe] …

The active site of the [FeFe]-hydrogenase from Desulfovibrio desulfuricans. II. Redox properties, light sensitivity and CO-ligand exchange as observed by infrared …

W Roseboom, AL De Lacey, VM Fernandez… - JBIC Journal of …, 2006 - Springer
Abstract In [FeFe]-hydrogenases, the H cluster (hydrogen-activating cluster) contains a di-
iron centre ([2Fe] H subcluster, a (L)(CO)(CN) Fe (μ-RS 2)(μ-CO) Fe (CysS)(CO)(CN) group) …

Catalysis of the electrochemical H2 evolution by di-iron sub-site models

JF Capon, F Gloaguen, P Schollhammer… - Coordination Chemistry …, 2005 - Elsevier
A short non-exhaustive overview of hexacarbonyl dithiolate di-iron species and of their
substituted derivatives relevant to the chemistry of the di-iron sub-site of the hydrogenase …

Iron-only hydrogenase: Synthetic, structural and reactivity studies of model compounds

X Liu, SK Ibrahim, C Tard, CJ Pickett - Coordination Chemistry Reviews, 2005 - Elsevier
Iron-only hydrogenase: Synthetic, structural and reactivity studies of model compounds -
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