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Electrochemical reduction of carbon dioxide to multicarbon (C 2+) products: challenges and perspectives
Electrocatalytic CO2 reduction has been developed as a promising and attractive strategy to
achieve carbon neutrality for sustainable chemical production. Among various reduction …
achieve carbon neutrality for sustainable chemical production. Among various reduction …
Local reaction environment in electrocatalysis
Beyond conventional electrocatalyst engineering, recent studies have unveiled the
effectiveness of manipulating the local reaction environment in enhancing the performance …
effectiveness of manipulating the local reaction environment in enhancing the performance …
Accelerating electrochemical CO2 reduction to multi-carbon products via asymmetric intermediate binding at confined nanointerfaces
Abstract Electrochemical CO2 reduction (CO2R) to ethylene and ethanol enables the long-
term storage of renewable electricity in valuable multi-carbon (C2+) chemicals. However …
term storage of renewable electricity in valuable multi-carbon (C2+) chemicals. However …
Coverage-driven selectivity switch from ethylene to acetate in high-rate CO2/CO electrolysis
Tuning catalyst microenvironments by electrolytes and organic modifications is effective in
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …
Surface hydroxide promotes CO2 electrolysis to ethylene in acidic conditions
Performing CO2 reduction in acidic conditions enables high single-pass CO2 conversion
efficiency. However, a faster kinetics of the hydrogen evolution reaction compared to CO2 …
efficiency. However, a faster kinetics of the hydrogen evolution reaction compared to CO2 …
Bifunctional ionomers for efficient co-electrolysis of CO2 and pure water towards ethylene production at industrial-scale current densities
W Li, Z Yin, Z Gao, G Wang, Z Li, F Wei, X Wei, H Peng… - Nature Energy, 2022 - nature.com
Many CO2 electrolysers under development use liquid electrolytes (KOH solutions, for
example), yet using solid-state polymer electrolytes can in principle improve efficiency and …
example), yet using solid-state polymer electrolytes can in principle improve efficiency and …
Regulating reconstruction of oxide-derived Cu for electrochemical CO2 reduction toward n-propanol
Oxide-derived copper (OD-Cu) is the most efficient and likely practical electrocatalyst for
CO2 reduction toward multicarbon products. However, the inevitable but poorly understood …
CO2 reduction toward multicarbon products. However, the inevitable but poorly understood …
CO2 electrolysis to multicarbon products in strong acid
Carbon dioxide electroreduction (CO2R) is being actively studied as a promising route to
convert carbon emissions to valuable chemicals and fuels. However, the fraction of input …
convert carbon emissions to valuable chemicals and fuels. However, the fraction of input …
Rational design of electrocatalytic carbon dioxide reduction for a zero-carbon network
Electrocatalytic CO2 reduction has attracted much attention for its potential application in
CO2 mitigation and fuel production. During the past two decades, the electrocatalytic …
CO2 mitigation and fuel production. During the past two decades, the electrocatalytic …
Modulating electric field distribution by alkali cations for CO2 electroreduction in strongly acidic medium
The reaction of carbon dioxide with hydroxide to form carbonate in near-neutral or alkaline
medium severely limits the energy and carbon efficiency of CO2 electroreduction. Here we …
medium severely limits the energy and carbon efficiency of CO2 electroreduction. Here we …