The angular momentum of molecules, or, equivalently, their rotation in three-dimensional
space, is ideally suited for quantum control. Molecular angular momentum is naturally …

Molecular alignment and orientation by laser fields has attracted significant attention in
recent years, mostly due to new capabilities to manipulate the molecular spatial …

We demonstrate an angular high-harmonic spectroscopy method to probe the spinning
dynamics of a molecular rotation wave packet in real time. With the excitation of two time …

We conducted a joint theoretical and experimental study to investigate the collisional
dissipation of molecular alignment. By comparing experimental measurements to the …

Direct imaging of molecular dynamics is a long-standing goal in physics and chemistry. As
an emerging tool, high-order-harmonic spectroscopy (HHS) enables accessing molecular …

We demonstrate a method to simultaneously measure the rotational temperature and pump
intensity in laser-induced molecular alignment by the time-resolved high harmonic …

An all-optical measurement of high-order fractional molecular echoes is demonstrated by
using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser …

The rotational dynamics of a molecule is sensitive to neighboring atoms or molecules, which
can be used to probe the intermolecular interactions in the gas phase. Here, we real-time …

We study the dynamics of rotational echoes in gas phase molecular ensembles and their
dependence on the delay and intensity of the excitation pulses. We explore the unique …

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique
which utilizes strong optical fields to resolve coherent electron dynamics spanning an …