Advances in catalytic enantioselective fluorination, mono-, di-, and trifluoromethylation, and trifluoromethylthiolation reactions

X Yang, T Wu, RJ Phipps, FD Toste - Chemical reviews, 2015 - ACS Publications
1. INTRODUCTION Despite being largely absent from natural products and biological
processes, fluorine plays a conspicuous and increasingly important role within …

Modern approaches for asymmetric construction of carbon–fluorine quaternary stereogenic centers: synthetic challenges and pharmaceutical needs

Y Zhu, J Han, J Wang, N Shibata, M Sodeoka… - Chemical …, 2018 - ACS Publications
New methods for preparation of tailor-made fluorine-containing compounds are in extremely
high demand in nearly every sector of chemical industry. The asymmetric construction of …

Monofluorination of organic compounds: 10 years of innovation

PA Champagne, J Desroches, JD Hamel… - Chemical …, 2015 - ACS Publications
Taking into account the vast arrays of fluorinated motifs known, 11 this review will be limited
to the monofluorination of organic compounds, ie, synthetic methods allowing the …

The development of multidimensional analysis tools for asymmetric catalysis and beyond

MS Sigman, KC Harper, EN Bess… - Accounts of chemical …, 2016 - ACS Publications
Conspectus In most modern organic chemistry reports, including many of ours, reaction
optimization schemes are typically presented to showcase how reaction conditions have …

Late-stage fluorination: fancy novelty or useful tool?

CN Neumann, T Ritter - Angewandte Chemie (International ed. in …, 2015 - europepmc.org
Charming fluorine: This Essay examines the recent surge in late-stage fluorination reactions
and outlines challenges that need to be overcome to increase the impact of modern …

The Deuterated “Magic Methyl” Group: A Guide to Site‐Selective Trideuteromethyl Incorporation and Labeling by Using CD3 Reagents

J Steverlynck, R Sitdikov… - Chemistry–A European …, 2021 - Wiley Online Library
In the field of medicinal chemistry, the precise installation of a trideuteromethyl group is
gaining ever‐increasing attention. Site‐selective incorporation of the deuterated “magic …

Addition and correction to complete field guide to asymmetric BINOL-phosphate derived Brønsted acid and metal catalysis: History and classification by mode of …

D Parmar, E Sugiono, S Raja, M Rue** - Chemical Reviews, 2017 - ACS Publications
Figure 73: The proposed catalyst/substrate interaction shown in Figure 73 corresponds to
the related sulfoxidation catalyzed by chiral phosphoric acid PA 5 (ref 133). Please note that …

Chiral Selenide-Catalyzed Enantioselective Allylic Reaction and Intermolecular Difunctionalization of Alkenes: Efficient Construction of C-SCF3 Stereogenic …

X Liu, Y Liang, J Ji, J Luo, X Zhao - Journal of the American …, 2018 - ACS Publications
New approaches for the synthesis of enantiopure trifluoromethylthiolated molecules by
chiral selenide-catalyzed allylic trifluoromethylthiolation and intermolecular …

Stereoselectivity and substrate specificity of the Fe (II)/α-ketoglutarate-dependent oxygenase TqaL

H Tao, R Ushimaru, T Awakawa, T Mori… - Journal of the …, 2022 - ACS Publications
Non-heme iron enzymes are versatile catalysts in the biosynthesis of medicinal natural
products and have attracted increasing attention as practical catalytic tools in chemical …

Catalytic dynamic kinetic resolutions in tandem to construct two-axis terphenyl atropisomers

OM Beleh, E Miller, FD Toste… - Journal of the American …, 2020 - ACS Publications
The defined structure of molecules bearing multiple stereogenic axes is of increasing
relevance to materials science, pharmaceuticals, and catalysis. However, catalytic …