Two-dimensional electronic spectroscopy

E Fresch, FVA Camargo, Q Shen, CC Bellora… - Nature Reviews …, 2023 - nature.com
Two-dimensional electronic spectroscopy (2DES) is a popular technique that can track
ultrafast coherent and incoherent processes in real time. Since its development in the late …

Coherent two-dimensional and broadband electronic spectroscopies

S Biswas, JW Kim, X Zhang, GD Scholes - Chemical Reviews, 2022 - ACS Publications
Over the past few decades, coherent broadband spectroscopy has been widely used to
improve our understanding of ultrafast processes (eg, photoinduced electron transfer, proton …

Vibronic coherence in oxygenic photosynthesis

FD Fuller, J Pan, A Gelzinis, V Butkus, SS Senlik… - Nature …, 2014 - nature.com
Photosynthesis powers life on our planet. The basic photosynthetic architecture consists of
antenna complexes that harvest solar energy and reaction centres that convert the energy …

Coherence in Chemistry: Foundations and Frontiers

JD Schultz, JL Yuly, EA Arsenault, K Parker… - Chemical …, 2024 - ACS Publications
Coherence refers to correlations in waves. Because matter has a wave-particle nature, it is
unsurprising that coherence has deep connections with the most contemporary issues in …

Experimental implementations of two-dimensional Fourier transform electronic spectroscopy

FD Fuller, JP Ogilvie - Annual review of physical chemistry, 2015 - annualreviews.org
Two-dimensional electronic spectroscopy (2DES) reveals connections between an optical
excitation at a given frequency and the signals it creates over a wide range of frequencies …

Higher-order multidimensional and pump–probe spectroscopies

J Lüttig, S Mueller, P Malý, JJ Krich… - The journal of physical …, 2023 - ACS Publications
Transient absorption and coherent two-dimensional spectroscopy are widely established
methods for the investigation of ultrafast dynamics in quantum systems. Conventionally, they …

Frequency combs enable rapid and high-resolution multidimensional coherent spectroscopy

B Lomsadze, ST Cundiff - Science, 2017 - science.org
Dual laser frequency combs can rapidly measure high-resolution linear absorption spectra.
However, one-dimensional linear techniques cannot distinguish the sources of resonances …

Charge separation in the photosystem II reaction center resolved by multispectral two-dimensional electronic spectroscopy

HH Nguyen, Y Song, EL Maret, Y Silori, R Willow… - Science …, 2023 - science.org
The photosystem II reaction center (PSII RC) performs the primary energy conversion steps
of oxygenic photosynthesis. While the PSII RC has been studied extensively, the similar time …

Tri-comb spectroscopy

B Lomsadze, BC Smith, ST Cundiff - Nature Photonics, 2018 - nature.com
Multidimensional coherent spectroscopy (MDCS), is a powerful method that enables the
measurement of homogeneous linewidths in inhomogenously broadened systems, many …

Vibronic structure of photosynthetic pigments probed by polarized two-dimensional electronic spectroscopy and ab initio calculations

Y Song, A Schubert, E Maret, RK Burdick… - Chemical …, 2019 - pubs.rsc.org
Bacteriochlorophyll a (Bchl a) and chlorophyll a (Chl a) play important roles as light
absorbers in photosynthetic antennae and participate in the initial charge-separation steps …