Design principles for strong and tough hydrogels

X Li, JP Gong - Nature Reviews Materials, 2024 - nature.com
Hydrogels are crosslinked polymer networks swollen with water. Owing to their soft and
water-containing nature, hydrogels are promising materials for applications in many fields …

Structuring and sha** of mechanically robust and functional hydrogels toward wearable and implantable applications

XQ Wang, AQ **e, P Cao, J Yang, WL Ong… - Advanced …, 2024 - Wiley Online Library
Hydrogels possess unique features such as softness, wetness, responsiveness, and
biocompatibility, making them highly suitable for biointegrated applications that have close …

Connective tissue inspired elastomer-based hydrogel for artificial skin via radiation-indued penetrating polymerization

Y Tian, Z Wang, S Cao, D Liu, Y Zhang, C Chen… - Nature …, 2024 - nature.com
Robust hydrogels offer a candidate for artificial skin of bionic robots, yet few hydrogels have
a comprehensive performance comparable to real human skin. Here, we present a general …

Constructing phase separation in polymer gels: Strategies, functions and applications

Z Wang, W Qiu, Q Zhang - Progress in Polymer Science, 2024 - Elsevier
Over the past decades, there has been a flourishing of phase-separated polymer gels.
Unlike traditional design methods that rely on chemical structure and polymer network …

Autonomous underwater adhesion driven by water-induced interfacial rearrangement

L Yao, C Lin, X Duan, X Ming, Z Chen, H Zhu… - Nature …, 2023 - nature.com
Underwater adhesives receive extensive attention due to their wide applications in marine
explorations and various related industries. However, current adhesives still suffer from …

Bioinspired multiphase composite gel materials: From controlled micro-phase separation to multiple functionalities

Y Yang, Y Ru, T Zhao, M Liu - Chem, 2023 - cell.com
Phase separation in living organisms is essential for the execution of biological functions, for
example, the formation of membrane-less organelles and the functionalization of …

Supramolecular polyelectrolyte hydrogel based on conjoined double-networks for multifunctional applications

WJ Yang, R Zhang, X Guo, R Ma, Z Liu… - Journal of Materials …, 2022 - pubs.rsc.org
Recently, the skin-biomimetic ionic conductive hydrogels have emerged as a competitive
alternative in soft electronics applications due to their excellent ionic conductivity and good …

Hofmeister Effect‐Assisted Facile One‐Pot Fabrication of Double Network Organohydrogels with Exceptional Multi‐Functions

D Yu, J Yi, S Zhu, Y Tang, Y Huang… - Advanced Functional …, 2024 - Wiley Online Library
Multi‐functional hydrogels have gained attention for their potential as smart materials in
diverse applications. However, most established design principles and fabrication methods …

Role of hierarchy structure on the mechanical adaptation of self-healing hydrogels under cyclic stretching

X Li, K Cui, Y Zheng, YN Ye, C Yu, W Yang… - Science …, 2023 - science.org
Soft materials with mechanical adaptability have substantial potential for various
applications in tissue engineering. Gaining a deep understanding of the structural evolution …

Anti-swelling conductive polyampholyte hydrogels via ionic complexations for underwater motion sensors and dynamic information storage

X Ming, Y Sheng, L Yao, X Li, Y Huang, H Zhu… - Chemical Engineering …, 2023 - Elsevier
Swelling of hydrogels in aquatic environment is ubiquitous but unfavorable for underwater
applications, which dramatically diminishes their mechanical properties. In this study, we …