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Emerging atomistic modeling methods for heterogeneous electrocatalysis
Heterogeneous electrocatalysis lies at the center of various technologies that could help
enable a sustainable future. However, its complexity makes it challenging to accurately and …
enable a sustainable future. However, its complexity makes it challenging to accurately and …
Different distributions of multi-carbon products in CO2 and CO electroreduction under practical reaction conditions
Product selectivity differences between the electroreduction of CO2 and CO under practical
current densities are a widely encountered phenomenon that is rarely emphasized or …
current densities are a widely encountered phenomenon that is rarely emphasized or …
Tafel slope plot as a tool to analyze electrocatalytic reactions
Kinetic and nonkinetic contributions to the Tafel slope value can be separated using a Tafel
slope plot, where a constant Tafel slope region indicates kinetic meaningfulness. Here, we …
slope plot, where a constant Tafel slope region indicates kinetic meaningfulness. Here, we …
Reactive capture and electrochemical conversion of CO 2 with ionic liquids and deep eutectic solvents
Ionic liquids (ILs) and deep eutectic solvents (DESs) have tremendous potential for reactive
capture and conversion (RCC) of CO2 due to their wide electrochemical stability window …
capture and conversion (RCC) of CO2 due to their wide electrochemical stability window …
Promoting CO2 Electroreduction to Multi‐Carbon Products by Hydrophobicity‐Induced Electro‐Kinetic Retardation
Advancing the performance of the Cu‐catalyzed electrochemical CO2 reduction reaction
(CO2RR) is crucial for its practical applications. Still, the wettable pristine Cu surface often …
(CO2RR) is crucial for its practical applications. Still, the wettable pristine Cu surface often …
A covalent molecular design enabling efficient CO2 reduction in strong acids
Molecular complexes are an important class of catalysts for the electrochemical carbon
dioxide reduction reaction (CO2RR). However, selective CO2RR in strong acids remains …
dioxide reduction reaction (CO2RR). However, selective CO2RR in strong acids remains …
Potassium ion modulation of the Cu electrode-electrolyte interface with ionomers enhances CO2 reduction to C2+ products
Ionomers have shown promise as organic coatings on Cu electrodes to increase the CO 2
reduction (CO 2 R) selectivity toward multi-carbon (C 2+) products. However, the effects of …
reduction (CO 2 R) selectivity toward multi-carbon (C 2+) products. However, the effects of …
Electrochemical CO2 Reduction in Acidic Electrolytes: Spectroscopic Evidence for Local pH Gradients
Inspired by recent advances in electrochemical CO2 reduction (CO2R) under acidic
conditions, herein we leverage in situ spectroscopy to inform the optimization of CO2R at …
conditions, herein we leverage in situ spectroscopy to inform the optimization of CO2R at …
Directing CO2 electroreduction pathways for selective C2 product formation using single-site doped copper catalysts
Manipulating the selectivity-determining step in post-C–C coupling is crucial for enhancing
C2 product specificity during electrocatalytic CO2 reduction, complementing efforts to boost …
C2 product specificity during electrocatalytic CO2 reduction, complementing efforts to boost …
CO2 Conversion to Butene via a Tandem Photovoltaic–Electrochemical/Photothermocatalytic Process: A Co-design Approach to Coupled Microenvironments
We developed a tandem, unassisted, solar-driven electrochemical and photothermocatalytic
process for the single-pass conversion of CO2 to butene using only simulated solar …
process for the single-pass conversion of CO2 to butene using only simulated solar …