Light–matter interaction at atomic scales

R Gutzler, M Garg, CR Ast, K Kuhnke, K Kern - Nature Reviews Physics, 2021 - nature.com
Light–matter interaction drives many systems, such as optoelectronic devices like light-
emitting diodes and solar cells, biological structures like photosystem II and potential future …

Creating designer quantum states of matter atom-by-atom

AA Khajetoorians, D Wegner, AF Otte, I Swart - Nature Reviews Physics, 2019 - nature.com
Advances in high-resolution and spin-resolved scanning tunnelling microscopy, as well as
atomic-scale manipulation, have enabled the bottom-up, atom-by-atom creation and …

A quantum sensor for atomic-scale electric and magnetic fields

T Esat, D Borodin, J Oh, AJ Heinrich, FS Tautz… - Nature …, 2024 - nature.com
The detection of faint magnetic fields from single-electron and nuclear spins at the atomic
scale is a long-standing challenge in physics. While current mobile quantum sensors …

Electron spin resonance of single iron phthalocyanine molecules and role of their non-localized spins in magnetic interactions

X Zhang, C Wolf, Y Wang, H Aubin, T Bilgeri… - Nature Chemistry, 2022 - nature.com
Electron spin resonance (ESR) spectroscopy is a crucial tool, through spin labelling, in
investigations of the chemical structure of materials and of the electronic structure of …

Reading and writing single-atom magnets

FD Natterer, K Yang, W Paul, P Willke, T Choi, T Greber… - Nature, 2017 - nature.com
The single-atom bit represents the ultimate limit of the classical approach to high-density
magnetic storage media. So far, the smallest individually addressable bistable magnetic bits …

Atomic-scale quantum sensing based on the ultrafast coherence of an H2 molecule in an STM cavity

L Wang, Y **a, W Ho - Science, 2022 - science.org
A scanning tunneling microscope (STM) combined with a pump-probe femtosecond
terahertz (THz) laser can enable coherence measurements of single molecules. We report …

Coherent spin control of single molecules on a surface

P Willke, T Bilgeri, X Zhang, Y Wang, C Wolf, H Aubin… - ACS …, 2021 - ACS Publications
Control of single electron spins constitutes one of the most promising platforms for
spintronics, quantum sensing, and quantum information processing. Utilizing single …

Spin-polarized Yu-Shiba-Rusinov states in an iron-based superconductor

D Wang, J Wiebe, R Zhong, G Gu, R Wiesendanger - Physical Review Letters, 2021 - APS
Yu-Shiba-Rusinov (YSR) bound states appear when a magnetic atom interacts with a
superconductor. Here, we report on spin-resolved spectroscopic studies of YSR states …

Free coherent evolution of a coupled atomic spin system initialized by electron scattering

LM Veldman, L Farinacci, R Rejali, R Broekhoven… - Science, 2021 - science.org
Full insight into the dynamics of a coupled quantum system depends on the ability to follow
the effect of a local excitation in real-time. Here, we trace the free coherent evolution of a pair …

Hyperfine interaction of individual atoms on a surface

P Willke, Y Bae, K Yang, JL Lado, A Ferrón, T Choi… - Science, 2018 - science.org
Taking advantage of nuclear spins for electronic structure analysis, magnetic resonance
imaging, and quantum devices hinges on knowledge and control of the surrounding atomic …