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Ultrafast electron diffraction: Visualizing dynamic states of matter
Since the discovery of electron-wave duality, electron scattering instrumentation has
developed into a powerful array of techniques for revealing the atomic structure of matter …
developed into a powerful array of techniques for revealing the atomic structure of matter …
Spontaneous oxidation in aqueous microdroplets: water radical cation as primary oxidizing agent
Exploration of the unique chemical properties of interfaces can unlock new understanding. A
striking example is the finding of accelerated reactions, particularly spontaneous oxidation …
striking example is the finding of accelerated reactions, particularly spontaneous oxidation …
A contact-electro-catalytic cathode recycling method for spent lithium-ion batteries
With the global trend towards carbon neutrality, the demand for lithium-ion batteries (LIBs) is
continuously increasing. However, current recycling methods for spent LIBs need urgent …
continuously increasing. However, current recycling methods for spent LIBs need urgent …
Three-dimensional nanofabrication via ultrafast laser patterning and kinetically regulated material assembly
A major challenge in nanotechnology is the fabrication of complex three-dimensional (3D)
structures with desired materials. We present a strategy for fabricating arbitrary 3D …
structures with desired materials. We present a strategy for fabricating arbitrary 3D …
Capture of hydroxyl radicals by hydronium cations in water microdroplets
Despite the high stability of bulk water, water microdroplets possess strikingly different
properties, such as the presence of hydroxyl radicals (OH⋅) at the air–water interface …
properties, such as the presence of hydroxyl radicals (OH⋅) at the air–water interface …
What controls the quality of photodynamical simulations? Electronic structure versus nonadiabatic algorithm
The field of nonadiabatic dynamics has matured over the last decade with a range of
algorithms and electronic structure methods available at the moment. While the community …
algorithms and electronic structure methods available at the moment. While the community …
The mutual neutralization of hydronium and hydroxide
Mutual neutralization of hydronium (H3O+) and hydroxide (OH−) ions is a very fundamental
chemical reaction. Yet, there is only limited experimental evidence about the underlying …
chemical reaction. Yet, there is only limited experimental evidence about the underlying …
Femtosecond electronic and hydrogen structural dynamics in ammonia imaged with ultrafast electron diffraction
Directly imaging structural dynamics involving hydrogen atoms by ultrafast diffraction
methods is complicated by their low scattering cross sections. Here we demonstrate that …
methods is complicated by their low scattering cross sections. Here we demonstrate that …
The birth and evolution of solvated electrons in the water
The photo-induced radiolysis of water is an elementary reaction in biology and chemistry,
forming solvated electrons, OH radicals, and hydronium cations on fast time scales. Here …
forming solvated electrons, OH radicals, and hydronium cations on fast time scales. Here …
Direct tracking of ultrafast proton transfer in water dimers
Upon ionization, water forms a highly acidic radical cation H2O+· that undergoes ultrafast
proton transfer (PT)—a pivotal step in water radiation chemistry, initiating the production of …
proton transfer (PT)—a pivotal step in water radiation chemistry, initiating the production of …