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Redox-and Charge-State Dependent Trends in 5, 6, and 7-Membered Boron Heterocycles: A Neutral Ligand Coordination Chemistry Approach to Boracyclic Cations …
Conspectus Boron heterocycles represent an important subset of heteroatom-incorporated
rings, attracting attention from organic, inorganic, and materials chemists. The empty pz …
rings, attracting attention from organic, inorganic, and materials chemists. The empty pz …
Unveiling Three Interconvertible Redox States of Boraphenalene
Neutral 1-boraphenalene displays the isoelectronic structure of the phenalenyl carbocation
and is expected to behave as an attractive organoboron multi-redox system. However, the …
and is expected to behave as an attractive organoboron multi-redox system. However, the …
Unlocking Biradical Character in Diborepins
Systems that possess open-and closed-shell behavior attract significant attention from
researchers due to their inherent redox and charge transport properties. Herein, we report …
researchers due to their inherent redox and charge transport properties. Herein, we report …
Silylene-Stabilized Neutral Dibora-Aromatics with a B═ B Bond
The unprecedented silylene-supported dibenzodiboraoxepin 2 and 9, 10-
diboraphenanthrene complexes 6 and 8 were synthesized. The (NHSi) 2B2 …
diboraphenanthrene complexes 6 and 8 were synthesized. The (NHSi) 2B2 …
Dianionic and Neutral Diboron-Centered Classical Diradicaloids
Herein, we report the syntheses and electronic structures of crystalline dianionic as well as
neutral diboron-centered classical diradicaloids as boron analogues of classical Thiele …
neutral diboron-centered classical diradicaloids as boron analogues of classical Thiele …
Topology-Directed Synthesis of Helical Phosphoniums with High Diradical Character and Polar-Dependent Electron Transfer
B Yang, S Yan, S Ban, Y Zhang, H Ma… - Chemistry of …, 2024 - ACS Publications
Molecular topology synthesis of polycyclic aromatic hydrocarbons (PAHs) with diradical
character takes root in intramolecular coupling breakthrough. Herein, we report selective Mn …
character takes root in intramolecular coupling breakthrough. Herein, we report selective Mn …
Borafluorene-Mediated Sulfur Activation: Isolation of Boryl-Linked S7 and S8 Catenates and Related Chalcogenide Molecules
Although the activation of elemental sulfur by main group compounds is well-documented in
the literature, the products of such reactions are often heterocyclic in nature. However, the …
the literature, the products of such reactions are often heterocyclic in nature. However, the …
Pentacyclic fused diborepinium ions with carbene-and carbone-mediated deep-blue to red emission
Designing molecules that can undergo late-stage modifications resulting in specific optical
properties is useful for develo** structure-function trends in materials, which ultimately …
properties is useful for develo** structure-function trends in materials, which ultimately …
Crystalline Radical Anion of a Diboratriazole and Its Conversion to a Neutral Radical Driven by a Carbene
One-electron reduction of diboratriazole 1 with potassium graphite (KC8) generates the
radical anion 1•–• K+, which undergoes a salt (KCl) elimination reaction upon addition of an …
radical anion 1•–• K+, which undergoes a salt (KCl) elimination reaction upon addition of an …
Silylene‐Copper‐Amide Emitters: From Thermally Activated Delayed Fluorescence to Dual Emission
Herein, we report the inaugural instance of N‐heterocyclic silylene (NHSi)‐coordinated
copper amide emitters (2–5). These complexes exhibit thermally activated delayed …
copper amide emitters (2–5). These complexes exhibit thermally activated delayed …