Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Enrichment of reactants and intermediates for electrocatalytic CO 2 reduction

PP Yang, MR Gao - Chemical Society Reviews, 2023 - pubs.rsc.org
The electrocatalytic carbon dioxide reduction reaction (CO2RR) presents a sustainable
route to convert renewable electricity to value-added fuels and feedstocks in the form of …

Coverage-driven selectivity switch from ethylene to acetate in high-rate CO2/CO electrolysis

P Wei, D Gao, T Liu, H Li, J Sang, C Wang… - Nature …, 2023 - nature.com
Tuning catalyst microenvironments by electrolytes and organic modifications is effective in
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …

Boosting electrocatalytic CO2–to–ethanol production via asymmetric C–C coupling

P Wang, H Yang, C Tang, Y Wu, Y Zheng… - Nature …, 2022 - nature.com
Electroreduction of carbon dioxide (CO2) into multicarbon products provides possibility of
large-scale chemicals production and is therefore of significant research and commercial …

Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction

J Wang, HY Tan, MY Qi, JY Li, ZR Tang… - Chemical Society …, 2023 - pubs.rsc.org
The ubiquity of solid–liquid interfaces in nature and the significant role of their atomic-scale
structure in determining interfacial properties have led to intensive research. Particularly in …

Amorphous Mo‐doped NiS0.5Se0.5 Nanosheets@Crystalline NiS0.5Se0.5 Nanorods for High Current‐density Electrocatalytic Water Splitting in Neutral Media

Y Wang, X Li, Z Huang, H Wang, Z Chen… - Angewandte Chemie …, 2023 - Wiley Online Library
It is vitally important to develop highly active, robust and low‐cost transition metal‐based
electrocatalysts for overall water splitting in neutral solution especially at large current …

Electrocatalytic CO2-to-C2+ with Ampere-Level Current on Heteroatom-Engineered Copper via Tuning *CO Intermediate Coverage

M Zheng, P Wang, X Zhi, K Yang, Y Jiao… - Journal of the …, 2022 - ACS Publications
An ampere-level current density of CO2 electrolysis is critical to realize the industrial
production of multicarbon (C2+) fuels. However, under such a large current density, the poor …

Membrane Electrode Assembly for Electrocatalytic CO2 Reduction: Principle and Application

Z Zhang, X Huang, Z Chen, J Zhu… - Angewandte …, 2023 - Wiley Online Library
Electrocatalytic CO2 reduction reaction (CO2RR) in membrane electrode assembly (MEA)
systems is a promising technology. Gaseous CO2 can be directly transported to the cathode …

Stabilizing Cu2+ Ions by Solid Solutions to Promote CO2 Electroreduction to Methane

X Zhou, J Shan, L Chen, BY **a, T Ling… - Journal of the …, 2022 - ACS Publications
Copper is the only metal catalyst that can perform the electrocatalytic CO2 reduction reaction
(CRR) to produce hydrocarbons and oxygenates. Its surface oxidation state determines the …

Electrochemical CO2 reduction (CO2RR) to multi-carbon products over copper-based catalysts

AR Woldu, Z Huang, P Zhao, L Hu, D Astruc - Coordination Chemistry …, 2022 - Elsevier
Copper has been recognized as the only heterogeneous catalyst leading to the formation of
various products of hydrocarbons and oxygenates, such as ethanol and ethylene, from the …