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Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …
carbon neutral through an alternative electrical approach to the energy-intensive …
Stability Issues in Electrochemical CO2 Reduction: Recent Advances in Fundamental Understanding and Design Strategies
Electrochemical CO2 reduction reaction (CO2RR) offers a promising approach to close the
anthropogenic carbon cycle and store intermittent renewable energy in fuels or chemicals …
anthropogenic carbon cycle and store intermittent renewable energy in fuels or chemicals …
In Situ Infrared Spectroscopic Evidence of Enhanced Electrochemical CO2 Reduction and C–C Coupling on Oxide-Derived Copper
The reaction mechanism of CO2 electroreduction on oxide-derived copper has not yet been
unraveled even though high C2+ Faradaic efficiencies are commonly observed on these …
unraveled even though high C2+ Faradaic efficiencies are commonly observed on these …
Solution-based Cu+ transient species mediate the reconstruction of copper electrocatalysts for CO2 reduction
J Vavra, GPL Ramona, F Dattila, A Kormányos… - Nature Catalysis, 2024 - nature.com
Understanding metal surface reconstruction is of the utmost importance in electrocatalysis,
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction
J Wang, HY Tan, MY Qi, JY Li, ZR Tang… - Chemical Society …, 2023 - pubs.rsc.org
The ubiquity of solid–liquid interfaces in nature and the significant role of their atomic-scale
structure in determining interfacial properties have led to intensive research. Particularly in …
structure in determining interfacial properties have led to intensive research. Particularly in …
Highly Efficient Electroreduction of CO2 to Ethanol via Asymmetric C–C Coupling by a Metal–Organic Framework with Heterodimetal Dual Sites
ZH Zhao, JR Huang, PQ Liao… - Journal of the American …, 2023 - ACS Publications
The electroreduction of CO2 into value-added liquid fuels holds great promise for
addressing global environmental and energy challenges. However, achieving highly …
addressing global environmental and energy challenges. However, achieving highly …
Steering the structure and selectivity of CO2 electroreduction catalysts by potential pulses
J Timoshenko, A Bergmann, C Rettenmaier, A Herzog… - Nature …, 2022 - nature.com
Convoluted selectivity trends and a missing link between reaction product distribution and
catalyst properties hinder practical applications of the electrochemical CO2 reduction …
catalyst properties hinder practical applications of the electrochemical CO2 reduction …
Identification of Cu(100)/Cu(111) Interfaces as Superior Active Sites for CO Dimerization During CO2 Electroreduction
The electrosynthesis of valuable multicarbon chemicals using carbon dioxide (CO2) as a
feedstock has substantially progressed recently but still faces considerable challenges. A …
feedstock has substantially progressed recently but still faces considerable challenges. A …
In situ copper faceting enables efficient CO2/CO electrolysis
The copper (Cu)-catalyzed electrochemical CO2 reduction provides a route for the synthesis
of multicarbon (C2+) products. However, the thermodynamically favorable Cu surface (ie Cu …
of multicarbon (C2+) products. However, the thermodynamically favorable Cu surface (ie Cu …
Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
The continuously increasing CO2 released from human activities poses a great threat to
human survival by fluctuating global climate and disturbing carbon balance among the four …
human survival by fluctuating global climate and disturbing carbon balance among the four …