Single-atom alloy catalysis

RT Hannagan, G Giannakakis… - Chemical …, 2020 - ACS Publications
Single-atom alloys (SAAs) play an increasingly significant role in the field of single-site
catalysis and are typically composed of catalytically active elements atomically dispersed in …

[HTML][HTML] Magic of hydrogen spillover: Understanding and application

H Shen, H Li, Z Yang, C Li - Green Energy & Environment, 2022 - Elsevier
The hydrogen spillover effect (HSPE) plays an important role in heterogeneous catalysis
and hydrogen storage as an interfacial phenomenon, which facilitates the improvement of …

Guidelines to achieving high selectivity for the hydrogenation of α, β-unsaturated aldehydes with bimetallic and dilute alloy catalysts: a review

M Luneau, JS Lim, DA Patel, ECH Sykes… - Chemical …, 2020 - ACS Publications
Selective hydrogenation of α, β-unsaturated aldehydes to unsaturated alcohols is a
challenging class of reactions, yielding valuable intermediates for the production of …

Single-atom alloys as a reductionist approach to the rational design of heterogeneous catalysts

G Giannakakis… - Accounts of chemical …, 2018 - ACS Publications
Conspectus Heterogeneous catalysts are workhorses in the industrial production of most
commodity and specialty chemicals, and have widespread energy and environmental …

Selective hydrogenation of 1, 3-butadiene on platinum–copper alloys at the single-atom limit

FR Lucci, J Liu, MD Marcinkowski, M Yang… - Nature …, 2015 - nature.com
Platinum is ubiquitous in the production sectors of chemicals and fuels; however, its scarcity
in nature and high price will limit future proliferation of platinum-catalysed reactions. One …

Isolated metal atom geometries as a strategy for selective heterogeneous hydrogenations

G Kyriakou, MB Boucher, AD Jewell, EA Lewis… - Science, 2012 - science.org
Facile dissociation of reactants and weak binding of intermediates are key requirements for
efficient and selective catalysis. However, these two variables are intimately linked in a way …

[書籍][B] Comprehensive handbook of chemical bond energies

YR Luo - 2007 - taylorfrancis.com
Understanding the energy it takes to build or break chemical bonds is essential for scientists
and engineers in a wide range of innovative fields, including catalysis, nanomaterials …

Reversible work transition state theory: application to dissociative adsorption of hydrogen

G Mills, H Jónsson, GK Schenter - Surface Science, 1995 - Elsevier
A practical method for finding free energy barriers for transitions in high-dimensional
classical and quantum systems is presented and used to calculate the dissociative sticking …

Quantum and thermal effects in dissociative adsorption: Evaluation of free energy barriers in multidimensional quantum systems

G Mills, H Jónsson - Physical review letters, 1994 - APS
We have evaluated the sticking probability and activation energy for dissociation of H 2
molecules on a Cu (110) surface by a reversible work formulation of quantum transition state …

Hydrogen adsorption, absorption and diffusion on and in transition metal surfaces: A DFT study

P Ferrin, S Kandoi, AU Nilekar, M Mavrikakis - Surface science, 2012 - Elsevier
Periodic, self-consistent DFT-GGA (PW91) calculations are used to study the interaction of
hydrogen with different facets of seventeen transition metals—the (100) and (111) facets of …