Exciton transport in molecular aggregates–from natural antennas to synthetic chromophore systems

T Brixner, R Hildner, J Köhler… - Advanced Energy …, 2017 - Wiley Online Library
The transport of excitation energy in molecular aggregates is of crucial importance for the
function of organic optoelectronic devices and next‐generation solar cells. First, this review …

[HTML][HTML] Two-dimensional spectroscopy for non-specialists

A Gelzinis, R Augulis, V Butkus, B Robert… - Biochimica et Biophysica …, 2019 - Elsevier
Detailed studies of the excitation dynamics in photosynthetic pigment-proteins require an
application of a wide range of spectroscopic methods. From the later part of the previous …

Energy relaxation pathways between light-matter states revealed by coherent two-dimensional spectroscopy

L Mewes, M Wang, RA Ingle, K Börjesson… - Communications …, 2020 - nature.com
Coupling matter excitations to electromagnetic modes inside nano-scale optical resonators
leads to the formation of hybrid light-matter states, so-called polaritons, allowing the …

Vibronic coupling in organic semiconductors for photovoltaics

A De Sio, C Lienau - Physical Chemistry Chemical Physics, 2017 - pubs.rsc.org
Light-induced charge transfer from the photoexcited donor to the acceptor is the
fundamental step towards current generation in organic solar cells. Experimental evidence …

Primary processes in the bacterial reaction center probed by two-dimensional electronic spectroscopy

A Niedringhaus, VR Policht, R Sechrist, A Konar… - Proceedings of the …, 2018 - pnas.org
In the initial steps of photosynthesis, reaction centers convert solar energy to stable charge-
separated states with near-unity quantum efficiency. The reaction center from purple …

From wavelike to sub-diffusive motion: exciton dynamics and interaction in squaraine copolymers of varying length

P Malý, J Lüttig, A Turkin, J Dostál, C Lambert… - Chemical …, 2020 - pubs.rsc.org
Exciton transport and exciton–exciton interactions in molecular aggregates and polymers
are of great importance in natural photosynthesis, organic electronics, and related areas of …

[HTML][HTML] Two-dimensional fluorescence excitation spectroscopy: A novel technique for monitoring excited-state photophysics of molecular species with high time and …

J Yang, MF Gelin, L Chen, F Šanda… - The Journal of …, 2023 - pubs.aip.org
We propose a novel UV/Vis femtosecond spectroscopic technique, two-dimensional
fluorescence-excitation (2D-FLEX) spectroscopy, which combines spectral resolution during …

High-order pump–probe and high-order two-dimensional electronic spectroscopy on the example of squaraine oligomers

J Lüttig, PA Rose, P Malý, A Turkin, M Bühler… - The Journal of …, 2023 - pubs.aip.org
Time-resolved spectroscopy is commonly used to study diverse phenomena in chemistry,
biology, and physics. Pump–probe experiments and coherent two-dimensional (2D) …

Extracting the frequency-dependent dynamic Stokes shift from two-dimensional electronic spectra with prominent vibrational coherences

J Lu, Y Lee, JM Anna - The Journal of Physical Chemistry B, 2020 - ACS Publications
The dynamic Stokes shift is a common means for characterizing ultrafast solvation dynamics
of electronically excited states. Here we extract the excitation frequency-dependent dynamic …

Broadband visible two-dimensional spectroscopy of molecular dyes

L Mewes, RA Ingle, A Al Haddad… - The Journal of Chemical …, 2021 - pubs.aip.org
Two-dimensional Fourier transform spectroscopy is a promising technique to study ultrafast
molecular dynamics. Similar to transient absorption spectroscopy, a more complete picture …