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Vibrational spectroscopy and dynamics of water
We present an overview of recent static and time-resolved vibrational spectroscopic studies
of liquid water from ambient conditions to the supercooled state, as well as of crystalline and …
of liquid water from ambient conditions to the supercooled state, as well as of crystalline and …
Water: A tale of two liquids
Water is the most abundant liquid on earth and also the substance with the largest number
of anomalies in its properties. It is a prerequisite for life and as such a most important subject …
of anomalies in its properties. It is a prerequisite for life and as such a most important subject …
Electrofreezing of liquid water at ambient conditions
Water is routinely exposed to external electric fields. Whether, for example, at physiological
conditions, in contact with biological systems, or at the interface of polar surfaces in …
conditions, in contact with biological systems, or at the interface of polar surfaces in …
Surface-sensitive and surface-specific ultrafast two-dimensional vibrational spectroscopy
Ultrafast two-dimensional infrared spectroscopy (2D IR) has been advanced in recent years
toward measuring signals from only a monolayer of sample molecules at solid–liquid and …
toward measuring signals from only a monolayer of sample molecules at solid–liquid and …
Two-dimensional Raman-terahertz spectroscopy of water
Two-dimensional Raman-terahertz (THz) spectroscopy is presented as a multidimensional
spectroscopy directly in the far-IR regime. The method is used to explore the dynamics of the …
spectroscopy directly in the far-IR regime. The method is used to explore the dynamics of the …
A liquid-liquid transition in supercooled aqueous solution related to the HDA-LDA transition
Simulations and theory suggest that the thermodynamic anomalies of water may be related
to a phase transition between two supercooled liquid states, but so far this phase transition …
to a phase transition between two supercooled liquid states, but so far this phase transition …
Coherent X-rays reveal the influence of cage effects on ultrafast water dynamics
The dynamics of liquid water feature a variety of time scales, ranging from extremely fast
ballistic-like thermal motion, to slower molecular diffusion and hydrogen-bond …
ballistic-like thermal motion, to slower molecular diffusion and hydrogen-bond …
Thermodynamics of supercooled and stretched water: Unifying two-structure description and liquid-vapor spinodal
We have applied a two-structure approach to the description of the thermodynamic
properties of supercooled and stretched water, metastable toward vapor, ice, or both, by …
properties of supercooled and stretched water, metastable toward vapor, ice, or both, by …
Collective hydrogen bond reorganization in water studied with temperature-dependent ultrafast infrared spectroscopy
We use temperature-dependent ultrafast infrared spectroscopy of dilute HOD in H2O to
study the picosecond reorganization of the hydrogen bond network of liquid water …
study the picosecond reorganization of the hydrogen bond network of liquid water …
[HTML][HTML] Multiple length and time scales of dynamic heterogeneities in model glass-forming liquids: A systematic analysis of multi-point and multi-time correlations
We report an extensive and systematic investigation of the multi-point and multi-time
correlation functions to reveal the spatio-temporal structures of dynamic heterogeneities in …
correlation functions to reveal the spatio-temporal structures of dynamic heterogeneities in …