Designing sites in heterogeneous catalysis: are we reaching selectivities competitive with those of homogeneous catalysts?

F Zaera - Chemical Reviews, 2022 - ACS Publications
A critical review of different prominent nanotechnologies adapted to catalysis is provided,
with focus on how they contribute to the improvement of selectivity in heterogeneous …

Surface organometallic chemistry in heterogeneous catalysis

MK Samantaray, E Pump… - Chemical Society …, 2018 - pubs.rsc.org
The broad challenges of energy and environment have become a main focus of research
efforts to develop more active and selective catalytic systems for key chemical …

Single‐atom catalysts supported on ordered porous materials: Synthetic strategies and applications

K Xue, Y Mo, B Long, W Wei, C Shan, S Guo, L Niu - InfoMat, 2022 - Wiley Online Library
Single‐atom catalysts (SACs) are attracting extensive attention due to their incredibly
catalytic activity and selectivity, high utilization of metal atoms, and obvious cost reduction …

Consequences of confinement for alkene epoxidation with hydrogen peroxide on highly dispersed group 4 and 5 metal oxide catalysts

DT Bregante, NE Thornburg, JM Notestein… - Acs …, 2018 - ACS Publications
Ti, Nb, and Ta atoms substituted into the framework of zeolite* BEA (M-BEA) or grafted onto
mesoporous silica (M-SiO2) irreversibly activate hydrogen peroxide (H2O2) to form pools of …

Periodic trends in olefin epoxidation over group IV and V framework-substituted zeolite catalysts: a kinetic and spectroscopic study

DT Bregante, DW Flaherty - Journal of the American Chemical …, 2017 - ACS Publications
Group IV and V framework-substituted zeolites have been used for olefin epoxidation
reactions for decades, yet the underlying properties that determine the selectivities and …

Alkene Epoxidations with H2O2 over Groups 4–6 Metal-Substituted BEA Zeolites: Reactive Intermediates, Reaction Pathways, and Linear Free-Energy …

EZ Ayla, DS Potts, DT Bregante, DW Flaherty - ACS Catalysis, 2020 - ACS Publications
Rates and selectivities for alkene epoxidations depend sensitively on the identity of the
active metal center for both heterogeneous and homogeneous catalysts. While group 6 …

Toward a Better Understanding of Intrinsic Activity Trends in Zr-Based Heterogeneous Catalysts for Meerwein–Pondorf–Verley Reduction of Levulinate Esters

X Yang, Z Yuan, M Zhou, F Chen, BQ Xu, H Shi - ACS Catalysis, 2023 - ACS Publications
Lewis acidic heterogeneous catalysts are known to be active for transfer hydrogenation of
carbonyl compounds, which occur naturally or can be derived from renewable feedstocks …

A review of the role of hydrogen peroxide in organic transformations

H Targhan, P Evans, K Bahrami - Journal of Industrial and Engineering …, 2021 - Elsevier
Under appropriate conditions, hydrogen peroxide is able to perform a multitude of oxidative
organic reactions in an economically, technically, and environmentally satisfying manner …

Metal organic frameworks as heterogeneous catalysts in olefin epoxidation and carbon dioxide cycloaddition

A Tombesi, C Pettinari - Inorganics, 2021 - mdpi.com
Metal–organic frameworks (MOFs) are a family of porous crystalline materials that serve in
some cases as versatile platforms for catalysis. In this review, we overview the recent …

Insight into pathways of methylene blue degradation with H2O2 over mono and bimetallic Nb, Zn oxides

L Wolski, M Ziolek - Applied Catalysis B: Environmental, 2018 - Elsevier
The aim of this work was to investigate the influence of surface properties of metal oxides
(Nb 2 O 5, ZnO and ZnNb 2 O 6) on the type of reactive oxygen species (ROS) formed in …