Decoherence of electron spins in nanoscale systems is important to quantum technologies
such as quantum information processing and magnetometry. It is also an ideal model …

Quantum information processing (QIP) could revolutionize areas ranging from chemical
modeling to cryptography. One key figure of merit for the smallest unit for QIP, the qubit, is …

A major challenge in using spins in the solid state for quantum technologies is protecting
them from sources of decoherence. This is particularly important in nanodevices where the …

The decoherence, or dephasing, of electron spins in paramagnetic molecules limits
sensitivity and resolution in electron paramagnetic resonance spectroscopy, and it …

We implemented the calculation of hyperfine tensors into such plane wave supercell code
working with the projector augmentation wave method that incorporates hybrid density …

We report a vanadium complex in a nuclear-spin free ligand field that displays two key
properties for an ideal candidate qubit system: long coherence times that persist at high …

Singlet fission describes the spin-conserving production of two triplet excitons from one
singlet exciton. The existence of a spin-2 (quintet) triplet-pair state as a product of singlet …

Nuclear spins serve as sensitive probes in chemistry and materials science and are
promising candidates for quantum information processing,,–. NMR, the resonant control of …

Sensing the internal dynamics of individual nuclear spins or clusters of nuclear spins has
recently become possible by observing the coherence decay of a nearby electronic spin: the …

In Er 3+: Y 2 SiO 5, we demonstrate the selective optical addressing of the Y 89 3+ nuclear
spins through their superhyperfine coupling with the Er 3+ electronic spins possessing large …