Machine learning for automated experimentation in scanning transmission electron microscopy

SV Kalinin, D Mukherjee, K Roccapriore… - npj Computational …, 2023 - nature.com
Abstract Machine learning (ML) has become critical for post-acquisition data analysis in
(scanning) transmission electron microscopy,(S) TEM, imaging and spectroscopy. An …

Probing electron beam induced transformations on a single-defect level via automated scanning transmission electron microscopy

KM Roccapriore, MG Boebinger, O Dyck, A Ghosh… - ACS …, 2022 - ACS Publications
A robust approach for real-time analysis of the scanning transmission electron microscopy
(STEM) data streams, based on ensemble learning and iterative training (ELIT) of deep …

Plasmon-enhanced fluorescence for biophotonics and bio-analytical applications

S Dasgupta, K Ray - Frontiers in Chemistry, 2024 - frontiersin.org
Fluorescence spectroscopy serves as an ultrasensitive sophisticated tool where background
noises which serve as a major impediment to the detection of the desired signals can be …

Physics discovery in nanoplasmonic systems via autonomous experiments in scanning transmission electron microscopy

KM Roccapriore, SV Kalinin, M Ziatdinov - Advanced Science, 2022 - Wiley Online Library
Physics‐driven discovery in an autonomous experiment has emerged as a dream
application of machine learning in physical sciences. Here, this work develops and …

Probe microscopy is all you need

SV Kalinin, R Vasudevan, Y Liu, A Ghosh… - Machine Learning …, 2023 - iopscience.iop.org
We pose that microscopy offers an ideal real-world experimental environment for the
development and deployment of active Bayesian and reinforcement learning methods …

A Platform for Atomic Fabrication and In Situ Synthesis in a Scanning Transmission Electron Microscope

O Dyck, AR Lupini, S Jesse - Small Methods, 2023 - Wiley Online Library
The engineering of quantum materials requires the development of tools able to address
various synthesis and characterization challenges. These include the establishment and …

Building Workflows for Interactive Human in the Loop Automated Experiment (hAE) in STEM-EELS

U Pratiush, KM Roccapriore, Y Liu, G Duscher… - arxiv preprint arxiv …, 2024 - arxiv.org
Exploring the structural, chemical, and physical properties of matter on the nano-and atomic
scales has become possible with the recent advances in aberration-corrected electron …