Computational approaches for XANES, VtC-XES, and RIXS using linear-response time-dependent density functional theory based methods

DR Nascimento, N Govind - Physical Chemistry Chemical Physics, 2022 - pubs.rsc.org
The emergence of state-of-the-art X-ray light sources has paved the way for novel
spectroscopies that take advantage of their atomic specificity to shed light on fundamental …

Multiscale electrostatic embedding simulations for modeling structure and dynamics of molecules in solution: a tutorial review

AO Dohn - International Journal of Quantum Chemistry, 2020 - Wiley Online Library
The main concepts and important technical details of electrostatic embedding quantum
mechanics/molecular mechanics (QM/MM) simulations are explained and illustrated with the …

Ferricyanide photo-aquation pathway revealed by combined femtosecond Kβ main line and valence-to-core x-ray emission spectroscopy

M Reinhard, A Gallo, M Guo, AT Garcia-Esparza… - Nature …, 2023 - nature.com
Reliably identifying short-lived chemical reaction intermediates is crucial to elucidate
reaction mechanisms but becomes particularly challenging when multiple transient species …

Photochemical and photophysical dynamics of the aqueous ferrate (VI) ion

C Antolini, CD Spellman Jr, CJ Otolski… - Journal of the …, 2022 - ACS Publications
Ferrate (VI) has the potential to play a key role in future water supplies. Its salts have been
suggested as “green” alternatives to current advanced oxidation and disinfection methods in …

Quantifying photoinduced polaronic distortions in inorganic lead halide perovskite nanocrystals

O Cannelli, N Colonna, M Puppin… - Journal of the …, 2021 - ACS Publications
The development of next-generation perovskite-based optoelectronic devices relies critically
on the understanding of the interaction between charge carriers and the polar lattice in out …

Ag (I)-Promoted Substitution of Cyanide from Hexacyanoferrate (II) with Pyrazine: A Kinetic and Mechanistic Study

A Srivastava, RM Naik, J Rai, A Asthana - Russian Journal of Physical …, 2021 - Springer
The kinetic spectrophotometric study of Ag (I)-promoted production of [Fe (CN) 5PZA] 3–was
performed by monitoring the absorbance at 440 nm, the λmax of yellow-colored complex [Fe …

Integrated quantum-classical protocol for the realistic description of solvated multinuclear mixed-valence transition-metal complexes and their solvatochromic …

G Prampolini, A Andersen, BI Poulter… - Journal of Chemical …, 2023 - ACS Publications
Linear cyanide-bridged polymetallic complexes, which undergo photoinduced metal-to-
metal charge transfer, represent prototypical systems for studying long-range electron …

Near-quantitative predictions of the first-shell coordination structure of hydrated first-row transition metal ions using K-edge X-ray absorption near-edge spectroscopy

S Ghosh, H Agarwal, M Galib, B Tran… - The Journal of …, 2022 - ACS Publications
The solvation structure of transition metal ions is important for applications in geochemistry,
biochemistry, energy storage, and environmental chemistry. We study the X-ray absorption …

[HTML][HTML] Solution phase high repetition rate laser pump x-ray probe picosecond hard x-ray spectroscopy at the Stanford Synchrotron Radiation Lightsource

M Reinhard, D Skoien, JA Spies… - Structural …, 2023 - pubs.aip.org
We present a dedicated end-station for solution phase high repetition rate (MHz) picosecond
hard x-ray spectroscopy at beamline 15-2 of the Stanford Synchrotron Radiation …

Manipulating valence and core electronic excitations of a transition-metal complex using UV/Vis and X-ray cavities

B Gu, SM Cavaletto, DR Nascimento, M Khalil… - Chemical …, 2021 - pubs.rsc.org
We demonstrate how optical cavities can be exploited to control both valence-and core-
excitations in a prototypical model transition metal complex, ferricyanide ([Fe (III)(CN) 6] 3−) …