Critical review on the degradation mechanisms and recent progress of Ni-rich layered oxide cathodes for lithium-ion batteries

Q Gan, N Qin, H Yuan, L Lu, Z Xu, Z Lu - EnergyChem, 2023 - Elsevier
Ni-rich layered transition metal oxides possess remarkably high capacity and thus are very
competitive cathode materials in high-energy lithium-ion batteries (LIBs) for electric vehicles …

Cracking vs. surface reactivity in high-nickel cathodes for lithium-ion batteries

S Lee, L Su, A Mesnier, Z Cui, A Manthiram - Joule, 2023 - cell.com
High-nickel layered oxide cathodes LiNi x Mn y Co z O 2 (NMC) experience microcracks
during cycling. This can expose fresh cathode surfaces for parasitic reactions and isolate …

Advances and perspectives in understanding the structure-redox relationship of layered Li-Co-Ni-Mn oxide cathode materials

Z Wang, L Li, Z Sun, P Tang, G Hu, J Tan, F Li - Progress in Materials …, 2024 - Elsevier
A comprehensive understanding of the relationship between the structure
(electron/bulk/surface structures) and redox chemistry in the cathodes was discussed in this …

[HTML][HTML] Deciphering and modulating energetics of solvation structure enables aggressive high-voltage chemistry of Li metal batteries

Z Wu, R Li, S Zhang, T Deng, H Zhang, R Zhang, J Liu… - Chem, 2023 - cell.com
The stability of localized high-concentrated electrolytes (LHCEs) on the Li metal anode has
been well established, but the understanding of its oxidation chemistry for high-voltage …

Factors Influencing Gas Evolution from High‐Nickel Layered Oxide Cathodes in Lithium‐Based Batteries

R Sim, A Manthiram - Advanced Energy Materials, 2024 - Wiley Online Library
Gas evolution from high‐nickel layered oxide cathodes (> 90% Ni) remains a major issue for
their practical application. Gaseous species, such as CO2, O2, and CO, that are evolved at …

Localized High‐Concentration Electrolytes with Low‐Cost Diluents Compatible with Both Cobalt‐Free LiNiO2 Cathode and Lithium‐Metal Anode

Z Guo, Z Cui, R Sim, A Manthiram - Small, 2023 - Wiley Online Library
High‐nickel layered oxide cathodes and lithium‐metal anode are promising candidates for
next‐generation battery systems due to their high energy density. Nevertheless, the …

Impact of dopants on suppressing gas evolution from high-nickel layered oxide cathodes

R Sim, Z Cui, A Manthiram - ACS Energy Letters, 2023 - ACS Publications
Gas release from high-Ni layered oxide cathodes (LiNi x Mn1-xyz Co y Al z O2; x> 0.8) can
jeopardize the overall performance and safety characteristics of the cell. A comprehensive …

Crossover effects in lithium‐metal batteries with a localized high concentration electrolyte and high‐nickel cathodes

J Langdon, A Manthiram - Advanced Materials, 2022 - Wiley Online Library
While crossover effects, such as transition‐metal dissolution, are well‐understood in lithium‐
ion batteries, there is a limited understanding of the effect of crossed‐over chemical species …

Protection of Cobalt-Free LiNiO2 from Degradation with Localized Saturated Electrolytes in Lithium-Metal Batteries

L Su, E Jo, A Manthiram - ACS Energy Letters, 2022 - ACS Publications
High-nickel layered oxide cathode materials are the most promising candidates for
develo** lithium-metal batteries (LMBs) because of their high energy density and low cost …

In situ interweaved binder framework mitigating the structural and interphasial degradations of High‐nickel cathodes in lithium‐ion batteries

B **, Z Cui, A Manthiram - Angewandte Chemie, 2023 - Wiley Online Library
The practical viability of high‐nickel layered oxide cathodes is compromised by the
interphasial and structural degradations. Herein, we demonstrate that by applying an in situ …