Oxide–and silicate–water interfaces and their roles in technology and the environment

JL Bañuelos, E Borguet, GE Brown Jr… - Chemical …, 2023 - ACS Publications
Interfacial reactions drive all elemental cycling on Earth and play pivotal roles in human
activities such as agriculture, water purification, energy production and storage …

Crystallization by particle attachment in synthetic, biogenic, and geologic environments

JJ De Yoreo, PUPA Gilbert, NAJM Sommerdijk… - Science, 2015 - science.org
BACKGROUND Numerous lines of evidence challenge the traditional interpretations of how
crystals nucleate and grow in synthetic and natural systems. In contrast to the monomer-by …

[HTML][HTML] Calcium phosphates in biomedical applications: materials for the future?

W Habraken, P Habibovic, M Epple, M Bohner - Materials today, 2016 - Elsevier
Our populations are aging. Some experts predict that 30% of hospital beds will soon be
occupied by osteoporosis patients. Statistics show that 20% of patients suffering from an …

Biomineralization: Integrating mechanism and evolutionary history

PUPA Gilbert, KD Bergmann, N Boekelheide… - Science …, 2022 - science.org
Calcium carbonate (CaCO3) biomineralizing organisms have played major roles in the
history of life and the global carbon cycle during the past 541 Ma. Both marine diversification …

Amorphous calcium carbonate particles form coral skeletons

T Mass, AJ Giuffre, CY Sun, CA Stifler… - Proceedings of the …, 2017 - National Acad Sciences
Do corals form their skeletons by precipitation from solution or by attachment of amorphous
precursor particles as observed in other minerals and biominerals? The classical model …

Microscopic structure of the polymer-induced liquid precursor for calcium carbonate

Y Xu, KCH Tijssen, PHH Bomans, A Akiva… - Nature …, 2018 - nature.com
Many biomineral crystals form complex non-equilibrium shapes, often via transient
amorphous precursors. Also in vitro crystals can be grown with non-equilibrium …

In situ mechanical reinforcement of polymer hydrogels via metal-coordinated crosslink mineralization

S Kim, AU Regitsky, J Song, J Ilavsky… - Nature …, 2021 - nature.com
Biological organic-inorganic materials remain a popular source of inspiration for bioinspired
materials design and engineering. Inspired by the self-assembling metal-reinforced mussel …

Designing solid materials from their solute state: a shift in paradigms toward a holistic approach in functional materials chemistry

D Gebauer, SE Wolf - Journal of the American Chemical Society, 2019 - ACS Publications
“Non-classical” notions consider formation pathways of crystalline materials where larger
species than monomeric chemical constituents, ie, ions or single molecules, play crucial …

Shape-preserving amorphous-to-crystalline transformation of CaCO3 revealed by in situ TEM

Z Liu, Z Zhang, Z Wang, B **, D Li… - Proceedings of the …, 2020 - National Acad Sciences
Organisms use inorganic ions and macromolecules to regulate crystallization from
amorphous precursors, endowing natural biominerals with complex morphologies and …

The crystallization of amorphous calcium carbonate is kinetically governed by ion impurities and water

M Albéric, L Bertinetti, Z Zou, P Fratzl… - Advanced …, 2018 - Wiley Online Library
Many organisms use amorphous calcium carbonate (ACC) and control its stability by various
additives and water; however, the underlying mechanisms are yet unclear. Here, the effect of …