Quantitative analysis of gas hydrates using Raman spectroscopy

J Qin, WF Kuhs - AIChE Journal, 2013 - Wiley Online Library
A calibration protocol to quantify the compositional information of gas hydrates using Raman
spectroscopy is proposed. Structure I pure CH4‐, CO2‐and C2H6‐hydrates in their …

DMSO hydration redefined: Unraveling the hydrophobic hydration of solutes with a mixed hydrophilic–hydrophobic characteristic

A Panuszko, P Bruździak, M Śmiechowski… - Journal of Molecular …, 2019 - Elsevier
Hydrophobic hydration of solutes with a mixed hydrophilic–hydrophobic characteristics is
still poorly understood. This is because both experimental and theoretical methods find it …

Catalytic activity of methanol in all-vapor subsecond clathrate-hydrate formation

JP Devlin - The Journal of Chemical Physics, 2014 - pubs.aip.org
Methanol's property as a catalyst in the formation of gas clathrate hydrates has been
recognized for several years and was recently employed in a broad ranging study [K. Shin …

[HTML][HTML] NH3 as unique non-classical content-former within clathrate hydrates

Z Maşlakcı, JP Devlin, N Uras-Aytemiz - The Journal of Chemical …, 2017 - pubs.aip.org
High quality FTIR spectra of aerosols of NH 3–THF and NH 3–TMO binary clathrate hydrates
(CHs) have been measured. Our recently developed all-vapor sub-second approach to …

NH3 as simple clathrate-hydrate catalyst: Experiment and theory

M Kılıç, JP Devlin, N Uras-Aytemiz - The Journal of chemical physics, 2018 - pubs.aip.org
The catalytic action of NH3 within the all-vapor approach for instant clathrate hydrate (CH)
formation is studied using both FTIR spectroscopy and ab initio molecular dynamics …

Transient translational and rotational water defects in gas hydrates

S Liang, D Liang, N Wu, L Yi, G Hu - The Journal of Physical …, 2017 - ACS Publications
We report our observations of the transient formation of the translational and rotational
defects in the host lattice of methane hydrates. We perform molecular dynamics simulations …

Tracking all-vapor instant gas-hydrate formation and guest molecule populations: A possible probe for molecules trapped in water nanodroplets

N Uras-Aytemiz, L Cwiklik, J Paul Devlin - The Journal of Chemical …, 2012 - pubs.aip.org
Quantitative Fourier-transform infrared spectra for low-temperature (160–200 K) aerosols of
clathrate-hydrate nanoparticles that contain large-cage catalysts and small-cage nonpolar …

H-bonding behavior of ethylene oxide within the clathrate hydrates revisited: Experiment and theory

Z Maşlakcı, JP Devlin, N Uras-Aytemiz - Chemical Physics Letters, 2020 - Elsevier
FTIR spectroscopy has been used to reexplore the nonclassical behavior of ethylene oxide
(EO) within the large cages of clathrate hydrates. In most of the spectroscopic studies of EO …

[HTML][HTML] Communication: Fourier-transform infrared probing of remarkable quantities of gas trapped in cold homogeneously nucleated nanodroplets

N Uras-Aytemiz, JP Devlin - The Journal of Chemical Physics, 2013 - pubs.aip.org
Studies of catalyzed all-vapor gas-hydrate formation on a sub-second timescale have been
extended with a special focus on liquid-droplet compositions at the instant of hydrate …

[HTML][HTML] CO2 and C2H2 in cold nanodroplets of oxygenated organic molecules and water

JP Devlin, F Balcı, Z Maşlakcı… - The Journal of Chemical …, 2014 - pubs.aip.org
Recent demonstrations of subsecond and microsecond timescales for formation of clathrate
hydrate nanocrystals hint at future methods of control of environmental and industrial gases …