Improving the accuracy of atomistic simulations of the electrochemical interface

R Sundararaman, D Vigil-Fowler, K Schwarz - Chemical reviews, 2022‏ - ACS Publications
Atomistic simulation of the electrochemical double layer is an ambitious undertaking,
requiring quantum mechanical description of electrons, phase space sampling of liquid …

How machine learning can accelerate electrocatalysis discovery and optimization

SN Steinmann, Q Wang, ZW Seh - Materials Horizons, 2023‏ - pubs.rsc.org
Advances in machine learning (ML) provide the means to bypass bottlenecks in the
discovery of new electrocatalysts using traditional approaches. In this review, we highlight …

Roadmap on ferroelectric hafnia-and zirconia-based materials and devices

JPB Silva, R Alcala, UE Avci, N Barrett, L Bégon-Lours… - APL Materials, 2023‏ - pubs.aip.org
Ferroelectric hafnium and zirconium oxides have undergone rapid scientific development
over the last decade, pushing them to the forefront of ultralow-power electronic systems …

How to validate machine-learned interatomic potentials

JD Morrow, JLA Gardner, VL Deringer - The Journal of chemical …, 2023‏ - pubs.aip.org
Machine learning (ML) approaches enable large-scale atomistic simulations with near-
quantum-mechanical accuracy. With the growing availability of these methods, there arises …

Combining machine learning and many-body calculations: coverage-dependent adsorption of CO on Rh (111)

P Liu, J Wang, N Avargues, C Verdi, A Singraber… - Physical Review Letters, 2023‏ - APS
Adsorption of carbon monoxide (CO) on transition-metal surfaces is a prototypical process in
surface sciences and catalysis. Despite its simplicity, it has posed great challenges to …

Kohn–Sham accuracy from orbital-free density functional theory via Δ-machine learning

S Kumar, X **g, JE Pask, AJ Medford… - The Journal of …, 2023‏ - pubs.aip.org
We present a Δ-machine learning model for obtaining Kohn–Sham accuracy from orbital-
free density functional theory (DFT) calculations. In particular, we employ a machine-learned …

Absolute standard hydrogen electrode potential and redox potentials of atoms and molecules: machine learning aided first principles calculations

R **nouchi, F Karsai, G Kresse - Chemical Science, 2025‏ - pubs.rsc.org
Constructing a self-consistent first-principles framework that accurately predicts the
properties of electron transfer reactions through finite-temperature molecular dynamics …

Data-efficient multifidelity training for high-fidelity machine learning interatomic potentials

J Kim, J Kim, J Kim, J Lee, Y Park… - Journal of the American …, 2024‏ - ACS Publications
Machine learning interatomic potentials (MLIPs) are used to estimate potential energy
surfaces (PES) from ab initio calculations, providing near-quantum-level accuracy with …

Machine-learned acceleration for molecular dynamics in CASTEP

TK Stenczel, Z El-Machachi, G Liepuoniute… - The Journal of …, 2023‏ - pubs.aip.org
Machine learning (ML) methods are of rapidly growing interest for materials modeling, and
yet, the use of ML interatomic potentials for new systems is often more demanding than that …

Quantum paraelectricity and structural phase transitions in strontium titanate beyond density functional theory

C Verdi, L Ranalli, C Franchini, G Kresse - Physical Review Materials, 2023‏ - APS
We demonstrate an approach for calculating temperature-dependent quantum and
anharmonic effects with beyond density-functional theory accuracy. By combining machine …