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[HTML][HTML] Diffusion-controlled reactions: an overview
DS Grebenkov - Molecules, 2023 - mdpi.com
We review the milestones in the century-long development of the theory of diffusion-
controlled reactions. Starting from the seminal work by von Smoluchowski, who recognized …
controlled reactions. Starting from the seminal work by von Smoluchowski, who recognized …
Extracting, quantifying, and comparing dynamical and biomechanical properties of living matter through single particle tracking
A panoply of new tools for tracking single particles and molecules has led to an explosion of
experimental data, leading to novel insights into physical properties of living matter …
experimental data, leading to novel insights into physical properties of living matter …
Paradigm shift in diffusion-mediated surface phenomena
DS Grebenkov - Physical Review Letters, 2020 - APS
Diffusion-mediated surface phenomena are crucial for human life and industry, with
examples ranging from oxygen capture by lung alveolar surface to heterogeneous catalysis …
examples ranging from oxygen capture by lung alveolar surface to heterogeneous catalysis …
Diffusion-limited reactions in dynamic heterogeneous media
Most biochemical reactions in living cells rely on diffusive search for target molecules or
regions in a heterogeneous overcrowded cytoplasmic medium. Rapid rearrangements of the …
regions in a heterogeneous overcrowded cytoplasmic medium. Rapid rearrangements of the …
Strong defocusing of molecular reaction times results from an interplay of geometry and reaction control
Textbook concepts of diffusion-versus kinetic-control are well-defined for reaction-kinetics
involving macroscopic concentrations of diffusive reactants that are adequately described by …
involving macroscopic concentrations of diffusive reactants that are adequately described by …
An encounter-based approach for restricted diffusion with a gradient drift
DS Grebenkov - Journal of Physics A: Mathematical and …, 2022 - iopscience.iop.org
We develop an encounter-based approach for describing restricted diffusion with a gradient
drift toward a partially reactive boundary. For this purpose, we introduce an extension of the …
drift toward a partially reactive boundary. For this purpose, we introduce an extension of the …
From single-particle stochastic kinetics to macroscopic reaction rates: fastest first-passage time of N random walkers
We consider the first-passage problem for N identical independent particles that are initially
released uniformly in a finite domain Ω and then diffuse toward a reactive area Γ, which can …
released uniformly in a finite domain Ω and then diffuse toward a reactive area Γ, which can …
Full distribution of first exit times in the narrow escape problem
In the scenario of the narrow escape problem (NEP) a particle diffuses in a finite container
and eventually leaves it through a small'escape window'in the otherwise impermeable …
and eventually leaves it through a small'escape window'in the otherwise impermeable …
Depletion of resources by a population of diffusing species
DS Grebenkov - Physical Review E, 2022 - APS
Depletion of natural and artificial resources is a fundamental problem and a potential cause
of economic crises, ecological catastrophes, and death of living organisms. Understanding …
of economic crises, ecological catastrophes, and death of living organisms. Understanding …
Redundancy principle and the role of extreme statistics in molecular and cellular biology
The paradigm of chemical activation rates in cellular biology has been shifted from the mean
arrival time of a single particle to the mean of the first among many particles to arrive at a …
arrival time of a single particle to the mean of the first among many particles to arrive at a …