Exact fundamental limits of the first and second hyperpolarizabilities

R Lytel, S Mossman, E Crowell, MG Kuzyk - Physical Review Letters, 2017 - APS
Nonlinear optical interactions of light with materials originate in the microscopic response of
the molecular constituents to excitation by an optical field, and are expressed by the first (β) …

Using excited states and degeneracies to enhance the electric polarizability and first hyperpolarizability

EL Crowell, MG Kuzyk - JOSA B, 2018 - opg.optica.org
We investigate the efficacy of boosting the nonlinear-optical response by using novel
systems such as those in an excited state or with a degenerate ground state. By applying the …

[KİTAP][B] Using Scale Invariance and the Fundamental Limits to Explore and Characterize Novel Enhancements of Optical Phenomena

EL Crowell - 2020 - search.proquest.com
Nonlinear optical phenomena promise profound impacts on science and technology.
However, materials with much larger nonlinear optical response are required before these …

[PDF][PDF] Ethan L. Crowell and Mark G. Kuzyk

F HYPERPOLARIZABILITY - USING SCALE INVARIANCE …, 2020 - rex.libraries.wsu.edu
The interaction of a material with an electric field is often well described by the electric
polarizability and hyperpolarizabilities. The polarizabilities derive from noting that the …

[KİTAP][B] Nonlinear optics near the fundamental limits

SM Mossman - 2017 - search.proquest.com
The nonlinear optical response of materials on the fastest time scale is ultimately determined
by the quantum mechanical properties of the material's electronic configuration. This …