Progress and prospects in nonlinear extreme-ultraviolet and X-ray optics and spectroscopy

M Chergui, M Beye, S Mukamel, C Svetina… - Nature Reviews …, 2023 - nature.com
Free-electron lasers and high-harmonic-generation table-top systems are new sources of
extreme-ultraviolet to hard X-ray photons, providing ultrashort pulses that are intense …

Experimental demonstration of attosecond pump–probe spectroscopy with an X-ray free-electron laser

Z Guo, T Driver, S Beauvarlet, D Cesar, J Duris… - Nature …, 2024 - nature.com
Pump–probe experiments with subfemtosecond resolution are the key to understanding
electronic dynamics in quantum systems. Here we demonstrate the generation and control …

Inverted nucleation for photoinduced nonequilibrium melting

J Hwang, Y Ihm, D Nam, J Shin, E Park, SY Lee… - Science …, 2024 - science.org
Ultrafast photoinduced melting provides an essential platform for studying nonequilibrium
phase transitions by linking the kinetics of electron dynamics to ionic motions. Knowledge of …

Few-femtosecond electron transfer dynamics in photoionized donor–π–acceptor molecules

F Vismarra, F Fernández-Villoria, D Mocci… - Nature Chemistry, 2024 - nature.com
The exposure of molecules to attosecond extreme-ultraviolet (XUV) pulses offers a unique
opportunity to study the early stages of coupled electron–nuclear dynamics in which the role …

Time-resolving state-specific molecular dissociation with XUV broadband absorption spectroscopy

A Magunia, M Rebholz, E Appi, CC Papadopoulou… - Science …, 2023 - science.org
The electronic and nuclear dynamics inside molecules are essential for chemical reactions,
where different pathways typically unfold on ultrafast timescales. Extreme ultraviolet (XUV) …

Core-hole coherent spectroscopy in molecules

E Rodríguez-Cuenca, A Picón, S Oberli, AI Kuleff… - Physical Review Letters, 2024 - APS
We study the ultrafast dynamics initiated by a coherent superposition of core-excited states
of nitrous oxide molecule. Using high-level ab initio methods, we show that the decoherence …

3D flower-like zinc do** engineered bismuth vanadium oxide architecture for boosted photocatalytic CO2 reduction to CH3OH

P Chang, H Yu, Y Zhang, Y Gao, L Zheng, K Li… - Journal of Molecular …, 2025 - Elsevier
Abstract Development of highly-efficient, selective, and durable CO 2 photocatalytic
reduction systems for high value-added carbon-containing chemicals or fuels is the key for …

Unraveling the electronic origin of a special feature in the triplet-minus-singlet spectra of carotenoids in natural photosystems

A Migliore, S Corni, A Agostini… - Physical Chemistry …, 2023 - pubs.rsc.org
The influence of carotenoid triplet states on the Qy electronic transitions of chlorophylls has
been observed in experiments on light-harvesting complexes over the past three decades …

Observation of molecular resonant double-core excitation driven by intense X-ray pulses

E Pelimanni, AEA Fouda, PJ Ho, TM Baumann… - Communications …, 2024 - nature.com
The ultrashort and intense pulses of X-rays produced at X-ray free electron lasers (XFELs)
have enabled unique experiments on the atomic level structure and dynamics of matter, with …

[HTML][HTML] X-ray induced electron and ion fragmentation dynamics in IBr

PJ Ho, D Ray, CS Lehmann, AEA Fouda… - The Journal of …, 2023 - pubs.aip.org
Characterization of the inner-shell decay processes in molecules containing heavy elements
is key to understanding x-ray damage of molecules and materials and for medical …