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[HTML][HTML] Charge migration and charge transfer in molecular systems
The transfer of charge at the molecular level plays a fundamental role in many areas of
chemistry, physics, biology and materials science. Today, more than 60 years after the …
chemistry, physics, biology and materials science. Today, more than 60 years after the …
Toward complete all-optical intensity modulation of high-harmonic generation from solids
Optical modulation of high-harmonics generation in solids enables the detection of material
properties, such as the band structure, and promising new applications, such as super …
properties, such as the band structure, and promising new applications, such as super …
Measurement and laser control of attosecond charge migration in ionized iodoacetylene
The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a
broad range of chemical and biophysical processes. We advanced high-harmonic …
broad range of chemical and biophysical processes. We advanced high-harmonic …
Chiral discrimination through bielliptical high-harmonic spectroscopy
Molecular chirality plays an essential role in most biochemical processes. The observation
and quantification of chirality-sensitive signals, however, remains extremely challenging …
and quantification of chirality-sensitive signals, however, remains extremely challenging …
Two-Center Interference in the Photoionization Delays of
We present the experimental observation of two-center interference in the ionization time
delays of Kr 2. Using attosecond electron-ion-coincidence spectroscopy, we simultaneously …
delays of Kr 2. Using attosecond electron-ion-coincidence spectroscopy, we simultaneously …
Two-pulse field-free orientation reveals anisotropy of molecular shape resonance
We report the observation of macroscopic field-free orientation, ie, more than 73% of CO
molecules pointing in the same direction. This is achieved through an all-optical scheme …
molecules pointing in the same direction. This is achieved through an all-optical scheme …
Channel coupling dynamics of deep-lying orbitals in molecular high-harmonic generation
Z Shu, H Liang, Y Wang, S Hu, S Chen, H Xu, R Ma… - Physical Review Letters, 2022 - APS
Investigation on structures in the high-harmonic spectrum has provided profuse information
of molecular structure and dynamics in intense laser fields, based on which techniques of …
of molecular structure and dynamics in intense laser fields, based on which techniques of …
Observation of laser-induced electronic structure in oriented polyatomic molecules
All attosecond time-resolved measurements have so far relied on the use of intense near-
infrared laser pulses. In particular, attosecond streaking, laser-induced electron diffraction …
infrared laser pulses. In particular, attosecond streaking, laser-induced electron diffraction …
Perspectives of attosecond spectroscopy for the understanding of fundamental electron correlations
The description of the electronic structure of molecules in terms of molecular orbitals is a
highly successful concept in chemistry. However, it commonly fails if the electrons in a …
highly successful concept in chemistry. However, it commonly fails if the electrons in a …
Strong-field approximation and its extension for high-order harmonic generation with mid-infrared lasers
In recent years intense mid-infrared lasers with wavelength of a few microns have become
the standard tools for research in strong field physics laboratories worldwide. These lasers …
the standard tools for research in strong field physics laboratories worldwide. These lasers …