[HTML][HTML] Charge migration and charge transfer in molecular systems

HJ Wörner, CA Arrell, N Banerji, A Cannizzo… - Structural …, 2017 - pubs.aip.org
The transfer of charge at the molecular level plays a fundamental role in many areas of
chemistry, physics, biology and materials science. Today, more than 60 years after the …

Toward complete all-optical intensity modulation of high-harmonic generation from solids

PJ van Essen, Z Nie, B de Keijzer, PM Kraus - ACS photonics, 2024 - ACS Publications
Optical modulation of high-harmonics generation in solids enables the detection of material
properties, such as the band structure, and promising new applications, such as super …

Measurement and laser control of attosecond charge migration in ionized iodoacetylene

PM Kraus, B Mignolet, D Baykusheva, A Rupenyan… - Science, 2015 - science.org
The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a
broad range of chemical and biophysical processes. We advanced high-harmonic …

Chiral discrimination through bielliptical high-harmonic spectroscopy

D Baykusheva, HJ Wörner - Physical Review X, 2018 - APS
Molecular chirality plays an essential role in most biochemical processes. The observation
and quantification of chirality-sensitive signals, however, remains extremely challenging …

Two-Center Interference in the Photoionization Delays of

S Heck, M Han, D Jelovina, JB Ji, C Perry, X Gong… - Physical review …, 2022 - APS
We present the experimental observation of two-center interference in the ionization time
delays of Kr 2. Using attosecond electron-ion-coincidence spectroscopy, we simultaneously …

Two-pulse field-free orientation reveals anisotropy of molecular shape resonance

PM Kraus, D Baykusheva, HJ Wörner - Physical review letters, 2014 - APS
We report the observation of macroscopic field-free orientation, ie, more than 73% of CO
molecules pointing in the same direction. This is achieved through an all-optical scheme …

Channel coupling dynamics of deep-lying orbitals in molecular high-harmonic generation

Z Shu, H Liang, Y Wang, S Hu, S Chen, H Xu, R Ma… - Physical Review Letters, 2022 - APS
Investigation on structures in the high-harmonic spectrum has provided profuse information
of molecular structure and dynamics in intense laser fields, based on which techniques of …

Observation of laser-induced electronic structure in oriented polyatomic molecules

PM Kraus, OI Tolstikhin, D Baykusheva… - Nature …, 2015 - nature.com
All attosecond time-resolved measurements have so far relied on the use of intense near-
infrared laser pulses. In particular, attosecond streaking, laser-induced electron diffraction …

Perspectives of attosecond spectroscopy for the understanding of fundamental electron correlations

PM Kraus, HJ Wörner - Angewandte Chemie International …, 2018 - Wiley Online Library
The description of the electronic structure of molecules in terms of molecular orbitals is a
highly successful concept in chemistry. However, it commonly fails if the electrons in a …

Strong-field approximation and its extension for high-order harmonic generation with mid-infrared lasers

AT Le, H Wei, C **, CD Lin - … of Physics B: Atomic, Molecular and …, 2016 - iopscience.iop.org
In recent years intense mid-infrared lasers with wavelength of a few microns have become
the standard tools for research in strong field physics laboratories worldwide. These lasers …