O2 Activation by Metal Surfaces: Implications for Bonding and Reactivity on Heterogeneous Catalysts

MM Montemore, MA Van Spronsen, RJ Madix… - Chemical …, 2017 - ACS Publications
The activation of O2 on metal surfaces is a critical process for heterogeneous catalysis and
materials oxidation. Fundamental studies of well-defined metal surfaces using a variety of …

Surface chemistry of ruthenium dioxide in heterogeneous catalysis and electrocatalysis: from fundamental to applied research

H Over - Chemical Reviews, 2012 - ACS Publications
Ruthenium is a chemical element that can easily adopt various formal oxidation states from−
II to+ VIII in chemical bonds,(1, 2) thus giving rise to many compounds with interesting and …

Catalytic combustion of methane over palladium-based catalysts

D Ciuparu, MR Lyubovsky, E Altman… - Catalysis …, 2002 - Taylor & Francis
Palladium-based catalysts are widely applied in exhaust catalytic converter and catalytic
combustion systems. The mechanism for methane oxidation on a Pd-based catalyst is …

Electrochemical behaviour of palladium electrode: Oxidation, electrodissolution and ionic adsorption

M Grdeń, M Łukaszewski, G Jerkiewicz, A Czerwiński - Electrochimica Acta, 2008 - Elsevier
In electrochemistry, Pourbaix diagrams also known as potential-pH diagrams map out the
regions of stability of metals as well as the regions of possible existence of stable …

Consequences of Metal–Oxide Interconversion for C–H Bond Activation during CH4 Reactions on Pd Catalysts

YH Chin, C Buda, M Neurock… - Journal of the American …, 2013 - ACS Publications
Mechanistic assessments based on kinetic and isotopic methods combined with density
functional theory are used to probe the diverse pathways by which C–H bonds in CH4 react …

Active sites and mechanisms for H2O2 decomposition over Pd catalysts

A Plauck, EE Stangland, JA Dumesic… - Proceedings of the …, 2016 - National Acad Sciences
A combination of periodic, self-consistent density functional theory (DFT-GGA-PW91)
calculations, reaction kinetics experiments on a SiO2-supported Pd catalyst, and mean-field …

Molecular beam experiments on model catalysts

J Libuda, HJ Freund - Surface Science Reports, 2005 - Elsevier
Heterogeneous catalysts are highly complex materials with respect to both their composition
and structure. The reaction kinetics on their surfaces is known to depend sensitively on …

Two-dimensional oxide on Pd (111)

E Lundgren, G Kresse, C Klein, M Borg, JN Andersen… - Physical Review Letters, 2002 - APS
The oxidation of Pd (111) leads to an incommensurate surface oxide, which was studied by
the use of scanning tunneling microscopy, surface x-ray diffraction, high resolution core level …

Surface chemistry of late transition metal oxides

JF Weaver - Chemical reviews, 2013 - ACS Publications
The surface chemistry of late transition metal oxides is scientifically interesting and can play
a central role in commercial applications of heterogeneous catalysis. The late transition …

Oscillatory CO oxidation on Pd (1 0 0) studied with in situ scanning tunneling microscopy

BLM Hendriksen, SC Bobaru, JWM Frenken - Surface Science, 2004 - Elsevier
We have studied the catalytic oxidation of CO on Pd (100) at atmospheric pressures, using a
combined flow reactor and scanning tunneling microscope (STM). By switching from a CO …