The transfer of charge at the molecular level plays a fundamental role in many areas of
chemistry, physics, biology and materials science. Today, more than 60 years after the …

Optical modulation of high-harmonics generation in solids enables the detection of material
properties, such as the band structure, and promising new applications, such as super …

The ultrafast motion of electrons and holes after light-matter interaction is fundamental to a
broad range of chemical and biophysical processes. We advanced high-harmonic …

We present a theoretical formalism for the calculation of attosecond delays in molecular
photoionization. It is shown how delays relevant to one-photon-ionization, also known as …

We report the observation of macroscopic field-free orientation, ie, more than 73% of CO
molecules pointing in the same direction. This is achieved through an all-optical scheme …

All attosecond time-resolved measurements have so far relied on the use of intense near-
infrared laser pulses. In particular, attosecond streaking, laser-induced electron diffraction …

The description of the electronic structure of molecules in terms of molecular orbitals is a
highly successful concept in chemistry. However, it commonly fails if the electrons in a …

The first high harmonic spectrum containing only the odd orders was observed in
experiments 30 years ago. However, a spectrum containing pure even harmonics has never …

Molecular orientation methods based on nonresonant two-color laser pulses having parallel
polarizations have been reported theoretically and experimentally. In this work, we …

Retrieving atomic and molecular properties from entangling macroscopic measurements is
an ambitious task. In particular, the phase difference between the adjacent attosecond …