Ultrafast spectroscopy: State of the art and open challenges

M Maiuri, M Garavelli, G Cerullo - Journal of the American …, 2019 - ACS Publications
Ultrafast spectroscopy techniques use sequences of ultrashort light pulses (with femto-to
attosecond durations) to study photoinduced dynamical processes in atoms, molecules …

Quantum design of photosynthesis for bio-inspired solar-energy conversion

E Romero, VI Novoderezhkin, R Van Grondelle - Nature, 2017 - nature.com
Photosynthesis is the natural process that converts solar photons into energy-rich products
that are needed to drive the biochemistry of life. Two ultrafast processes form the basis of …

All-mode quantum–classical path integral simulation of bacteriochlorophyll dimer exciton-vibration dynamics

A Bose, N Makri - The Journal of Physical Chemistry B, 2020 - ACS Publications
We use the quantum–classical path integral (QCPI) methodology to report numerically exact,
fully quantum mechanical results for the exciton-vibration dynamics in the …

Quantum biology: An update and perspective

Y Kim, F Bertagna, EM D'souza, DJ Heyes… - Quantum …, 2021 - mdpi.com
Understanding the rules of life is one of the most important scientific endeavours and has
revolutionised both biology and biotechnology. Remarkable advances in observation …

Quantum coherence in photosynthesis for efficient solar-energy conversion

E Romero, R Augulis, VI Novoderezhkin, M Ferretti… - Nature physics, 2014 - nature.com
The crucial step in the conversion of solar to chemical energy in photosynthesis takes place
in the reaction centre, where the absorbed excitation energy is converted into a stable …

Lessons from nature about solar light harvesting

GD Scholes, GR Fleming, A Olaya-Castro… - Nature …, 2011 - nature.com
Solar fuel production often starts with the energy from light being absorbed by an assembly
of molecules; this electronic excitation is subsequently transferred to a suitable acceptor. For …

Quantum chemical studies of light harvesting

C Curutchet, B Mennucci - Chemical reviews, 2017 - ACS Publications
The design of optimal light-harvesting (supra) molecular systems and materials is one of the
most challenging frontiers of science. Theoretical methods and computational models play a …

Structure and energy transfer in photosystems of oxygenic photosynthesis

N Nelson, W Junge - Annual review of biochemistry, 2015 - annualreviews.org
Oxygenic photosynthesis is the principal converter of sunlight into chemical energy on Earth.
Cyanobacteria and plants provide the oxygen, food, fuel, fibers, and platform chemicals for …

The role of non-equilibrium vibrational structures in electronic coherence and recoherence in pigment–protein complexes

AW Chin, J Prior, R Rosenbach, F Caycedo-Soler… - Nature Physics, 2013 - nature.com
Recent observations of oscillatory features in the optical response of photosynthetic
complexes have revealed evidence for surprisingly long-lasting electronic coherences …

Long-lived quantum coherence in photosynthetic complexes at physiological temperature

G Panitchayangkoon, D Hayes, KA Fransted… - Proceedings of the …, 2010 - pnas.org
Photosynthetic antenna complexes capture and concentrate solar radiation by transferring
the excitation to the reaction center that stores energy from the photon in chemical bonds …