Quantum computational chemistry

S McArdle, S Endo, A Aspuru-Guzik, SC Benjamin… - Reviews of Modern …, 2020 - APS
One of the most promising suggested applications of quantum computing is solving
classically intractable chemistry problems. This may help to answer unresolved questions …

Challenges for density functional theory

AJ Cohen, P Mori-Sánchez, W Yang - Chemical reviews, 2012 - ACS Publications
Density functional theory (DFT) of electronic structure has made an unparalleled impact on
the application of quantum mechanics to interesting and challenging problems in chemistry …

Long-range corrected hybrid density functionals with damped atom–atom dispersion corrections

JD Chai, M Head-Gordon - Physical Chemistry Chemical Physics, 2008 - pubs.rsc.org
We report re-optimization of a recently proposed long-range corrected (LC) hybrid density
functional [J.-D. Chai and M. Head-Gordon, J. Chem. Phys., 2008, 128, 084106] to include …

Density‐functional thermochemistry. I. The effect of the exchange‐only gradient correction

AD Becke - The Journal of chemical physics, 1992 - pubs.aip.org
Previous work by the author on diatomic molecules and by others on polyatomic systems
has revealed that Kohn–Sham density‐functional theory with ''gradient corrected''exchange …

A new mixing of Hartree–Fock and local density‐functional theories

AD Becke - The Journal of chemical physics, 1993 - pubs.aip.org
Previous attempts to combine Hartree-Fock theory with local density-functional theory have
been unsuccessful in applications to molecular bonding. We derive a new coupling of these …

Generalized gradient approximation made simple

JP Perdew, K Burke, M Ernzerhof - Physical review letters, 1996 - APS
Generalized gradient approximations (GGA's) for the exchange-correlation energy improve
upon the local spin density (LSD) description of atoms, molecules, and solids. We present a …

Rationale for mixing exact exchange with density functional approximations

JP Perdew, M Ernzerhof, K Burke - The Journal of chemical physics, 1996 - pubs.aip.org
Density functional approximations for the exchange-correlation energy Exc DFA of an
electronic system are often improved by admixing some exact exchange Ex: Exc Exc DFA …

Assessment of the Perdew–Burke–Ernzerhof exchange-correlation functional

M Ernzerhof, GE Scuseria - The Journal of chemical physics, 1999 - pubs.aip.org
In order to discriminate between approximations to the exchange-correlation energy E XC
[ρ↑, ρ↓], we employ the criterion of whether the functional is fitted to a certain experimental …

[HTML][HTML] The ONIOM method and its applications

LW Chung, WMC Sameera, R Ramozzi… - Chemical …, 2015 - ACS Publications
The fields of theoretical and computational chemistry have come a long way since their
inception in the mid-20th century. Fifty years ago, only rudimentary approximations for very …

Systematic optimization of long-range corrected hybrid density functionals

JD Chai, M Head-Gordon - The Journal of chemical physics, 2008 - pubs.aip.org
A general scheme for systematically modeling long-range corrected (LC) hybrid density
functionals is proposed. Our resulting two LC hybrid functionals are shown to be accurate in …