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Oxide–and silicate–water interfaces and their roles in technology and the environment
Interfacial reactions drive all elemental cycling on Earth and play pivotal roles in human
activities such as agriculture, water purification, energy production and storage …
activities such as agriculture, water purification, energy production and storage …
Water at charged interfaces
The ubiquity of aqueous solutions in contact with charged surfaces and the realization that
the molecular-level details of water–surface interactions often determine interfacial functions …
the molecular-level details of water–surface interactions often determine interfacial functions …
Multiscale modeling of aqueous electric double layers
From the stability of colloidal suspensions to the charging of electrodes, electric double
layers play a pivotal role in aqueous systems. The interactions between interfaces, water …
layers play a pivotal role in aqueous systems. The interactions between interfaces, water …
Water structure in the electrical double layer and the contributions to the total interfacial potential at different surface charge densities
The electric double layer governs the processes of all charged surfaces in aqueous
solutions; however, elucidating the structure of the water molecules is challenging for even …
solutions; however, elucidating the structure of the water molecules is challenging for even …
Uncovering the dominant role of an extended asymmetric four-coordinated water network in the hydrogen evolution reaction
S Li, L Wu, Q Liu, M Zhu, Z Li, C Wang… - Journal of the …, 2023 - ACS Publications
In situ and accurate measurement of the structure and dynamics of interfacial water in the
hydrogen evolution reaction (HER) is a well-known challenge because of the coupling of …
hydrogen evolution reaction (HER) is a well-known challenge because of the coupling of …
Elucidation of the pH-dependent electric double layer structure at the silica/water interface using heterodyne-detected vibrational sum frequency generation …
The silica/water interface is one of the most abundant charged interfaces in natural
environments, and the elucidation of the water structure at the silica/water interface is …
environments, and the elucidation of the water structure at the silica/water interface is …
Nature of cations critically affects water at the negatively charged silica interface
Understanding the collective behavior of ions at charged surfaces is of paramount
importance for geological and electrochemical processes. Ions screen the surface charge …
importance for geological and electrochemical processes. Ions screen the surface charge …
Probing the mineral–water interface with nonlinear optical spectroscopy
The interaction between minerals and water is manifold and complex: the mineral surface
can be (de) protonated by water, thereby changing its charge; mineral ions dissolved into …
can be (de) protonated by water, thereby changing its charge; mineral ions dissolved into …
The Solvation-Induced Onsager Reaction Field Rather than the Double-Layer Field Controls CO2 Reduction on Gold
The selectivity and activity of the carbon dioxide reduction (CO2R) reaction are sensitive
functions of the electrolyte cation. By measuring the vibrational Stark shift of in situ …
functions of the electrolyte cation. By measuring the vibrational Stark shift of in situ …
Ions tune interfacial water structure and modulate hydrophobic interactions at silica surfaces
The structure and ultrafast dynamics of the electric double layer (EDL) are central to
chemical reactivity and physical properties at solid/aqueous interfaces. While the Gouy …
chemical reactivity and physical properties at solid/aqueous interfaces. While the Gouy …