Progress and prospects in nonlinear extreme-ultraviolet and X-ray optics and spectroscopy

M Chergui, M Beye, S Mukamel, C Svetina… - Nature Reviews …, 2023 - nature.com
Free-electron lasers and high-harmonic-generation table-top systems are new sources of
extreme-ultraviolet to hard X-ray photons, providing ultrashort pulses that are intense …

Molecular chirality and its monitoring by ultrafast x-ray pulses

JR Rouxel, S Mukamel - Chemical Reviews, 2022 - ACS Publications
Major advances in X-ray sources including the development of circularly polarized and
orbital angular momentum pulses make it possible to probe matter chirality at …

Terawatt-scale attosecond X-ray pulses from a cascaded superradiant free-electron laser

P Franz, S Li, T Driver, RR Robles, D Cesar, E Isele… - Nature …, 2024 - nature.com
Intense attosecond X-ray pulses are key for ultrafast nonlinear spectroscopy and diffractive
imaging. Here we demonstrate the generation of terawatt-scale isolated attosecond pulses …

Experimental demonstration of attosecond pump–probe spectroscopy with an X-ray free-electron laser

Z Guo, T Driver, S Beauvarlet, D Cesar, J Duris… - Nature …, 2024 - nature.com
Pump–probe experiments with subfemtosecond resolution are the key to understanding
electronic dynamics in quantum systems. Here we demonstrate the generation and control …

Attosecond technology (ies) and science

J Biegert, F Calegari, N Dudovich… - Journal of Physics B …, 2021 - iopscience.iop.org
Since 2001 and the first demonstrations of the feasibility of generating and measuring
attosecond light pulses, attosecond science has developed into a very active and quickly …

Observation of site-selective chemical bond changes via ultrafast chemical shifts

A Al-Haddad, S Oberli, J González-Vázquez… - Nature …, 2022 - nature.com
The concomitant motion of electrons and nuclei on the femtosecond time scale marks the
fate of chemical and biological processes. Here we demonstrate the ability to initiate and …

Attosecond investigation of extreme-ultraviolet multi-photon multi-electron ionization

M Kretschmar, A Hadjipittas, B Major, J Tümmler, I Will… - Optica, 2022 - opg.optica.org
Multi-<? TeX 2pc 0pt?> electron<? TeX 4pc 0pt?> dynamics in atoms and molecules very
often occur on sub-to few-femtosecond time scales. The available intensities of extreme …

Time-resolved experiments on gas-phase atoms and molecules with XUV and X-ray free-electron lasers

D Rolles - Advances in Physics: X, 2023 - Taylor & Francis
Over the last 20 years, XUV and X-ray free-electron lasers have enabled a wide variety of
time-resolved experiments that have dramatically advanced our understanding of ultrafast …

Attosecond impulsive stimulated X-ray Raman scattering in liquid water

O Alexander, F Egun, L Rego, AM Gutierrez… - Science …, 2024 - science.org
We report the measurement of impulsive stimulated x-ray Raman scattering in neutral liquid
water. An attosecond pulse drives the excitations of an electronic wavepacket in water …

Controllable x-ray pulse trains from enhanced self-amplified spontaneous emission

JP Duris, JP MacArthur, JM Glownia, S Li, S Vetter… - Physical Review Letters, 2021 - APS
We report the demonstration of optical compression of an electron beam and the production
of controllable trains of femtosecond, soft x-ray pulses with the Linac Coherent Light Source …