Coherent two-dimensional and broadband electronic spectroscopies

S Biswas, JW Kim, X Zhang, GD Scholes - Chemical Reviews, 2022 - ACS Publications
Over the past few decades, coherent broadband spectroscopy has been widely used to
improve our understanding of ultrafast processes (eg, photoinduced electron transfer, proton …

Experimental implementations of two-dimensional Fourier transform electronic spectroscopy

FD Fuller, JP Ogilvie - Annual review of physical chemistry, 2015 - annualreviews.org
Two-dimensional electronic spectroscopy (2DES) reveals connections between an optical
excitation at a given frequency and the signals it creates over a wide range of frequencies …

Intrinsic homogeneous linewidth and broadening mechanisms of excitons in monolayer transition metal dichalcogenides

G Moody, C Kavir Dass, K Hao, CH Chen, LJ Li… - Nature …, 2015 - nature.com
The band-edge optical response of transition metal dichalcogenides, an emerging class of
atomically thin semiconductors, is dominated by tightly bound excitons localized at the …

Direct measurement of exciton valley coherence in monolayer WSe2

K Hao, G Moody, F Wu, CK Dass, L Xu, CH Chen… - Nature Physics, 2016 - nature.com
In crystals, energy band extrema in momentum space can be identified by a valley index.
The internal quantum degree of freedom associated with valley pseudospin indices can act …

Neutral and charged inter-valley biexcitons in monolayer MoSe2

K Hao, JF Specht, P Nagler, L Xu, K Tran… - Nature …, 2017 - nature.com
In atomically thin transition metal dichalcogenides (TMDs), reduced dielectric screening of
the Coulomb interaction leads to strongly correlated many-body states, including excitons …

Multidimensional coherent photocurrent spectroscopy of a semiconductor nanostructure

G Nardin, TM Autry, KL Silverman, ST Cundiff - Optics express, 2013 - opg.optica.org
Multidimensional Coherent Optical Photocurrent Spectroscopy (MD-COPS) is implemented
using unstabilized interferometers. Photocurrent from a semiconductor sample is generated …

Quantitative investigations of quantum coherence for a light-harvesting protein at conditions simulating photosynthesis

DB Turner, R Dinshaw, KK Lee, MS Belsley… - Physical Chemistry …, 2012 - pubs.rsc.org
Recent measurements using two-dimensional electronic spectroscopy (2D ES) have shown
that the initial dynamic response of photosynthetic proteins can involve quantum coherence …

Entangled two-photon absorption by atoms and molecules: A quantum optics tutorial

MG Raymer, T Landes, AH Marcus - The Journal of Chemical Physics, 2021 - pubs.aip.org
Two-photon absorption (TPA) and other nonlinear interactions of molecules with time–
frequency-entangled photon pairs have been predicted to display a variety of fascinating …

Multidimensional electronic spectroscopy of photochemical reactions

P Nuernberger, S Ruetzel… - Angewandte Chemie …, 2015 - Wiley Online Library
Coherent multidimensional electronic spectroscopy can be employed to unravel various
channels in molecular chemical reactions. This approach is thus not limited to analysis of …

Resonance lineshapes in two-dimensional Fourier transform spectroscopy

ME Siemens, G Moody, H Li, AD Bristow, ST Cundiff - Optics express, 2010 - opg.optica.org
We derive an analytical form for resonance lineshapes in two-dimensional (2D) Fourier
transform spectroscopy. Our starting point is the solution of the optical Bloch equations for a …