Controlling structure and properties of vapor-deposited glasses of organic semiconductors: Recent advances and challenges

K Bagchi, MD Ediger - The Journal of Physical Chemistry Letters, 2020 - ACS Publications
The past decade has seen great progress in manipulating the structure of vapor-deposited
glasses of organic semiconductors. Upon varying the substrate temperature during …

Anisotropic vapor-deposited glasses: hybrid organic solids

MD Ediger, J De Pablo, L Yu - Accounts of chemical research, 2019 - ACS Publications
Conspectus The term “organic solids” encompasses both crystals and glasses. Organic
crystals are commonly grown for purification and structure determination and are being …

MAIRS: Innovation of molecular orientation analysis in a thin film

T Hasegawa, N Shioya - Bulletin of the Chemical Society of …, 2020 - academic.oup.com
Multiple-angle incidence resolution spectrometry (MAIRS), originally developed in our
group, is a unique spectroscopic technique for analyzing the structure of molecular …

Origin of anisotropic molecular packing in vapor-deposited Alq3 glasses

K Bagchi, NE Jackson, A Gujral, C Huang… - The journal of …, 2018 - ACS Publications
Anisotropic molecular packing is a key feature that makes glasses prepared by physical
vapor deposition (PVD) unique materials, warranting a mechanistic understanding of how a …

Vapor-deposited glass structure determined by deposition rate–substrate temperature superposition principle

C Bishop, A Gujral, MF Toney, L Yu… - The journal of physical …, 2019 - ACS Publications
We show that deposition rate substantially affects the anisotropic structure of thin glassy
films produced by physical vapor deposition. Itraconazole, a glass-forming liquid crystal, was …

Using deposition rate and substrate temperature to manipulate liquid crystal-like order in a vapor-deposited hexagonal columnar glass

C Bishop, Z Chen, MF Toney, H Bock… - The Journal of …, 2021 - ACS Publications
We investigate vapor-deposited glasses of a phenanthroperylene ester, known to form an
equilibrium hexagonal columnar phase, and show that liquid crystal-like order can be …

Organic glasses with tunable liquid-crystalline order

R Teerakapibal, C Huang, A Gujral, MD Ediger, L Yu - Physical review letters, 2018 - APS
Liquid crystals (LCs) are known to undergo rapid ordering transitions with virtually no
hysteresis. We report a remarkable counterexample, itraconazole, where the nematic to …

Deep blue fluorescent material with an extremely high ratio of horizontal orientation to enhance light outcoupling efficiency (44%) and external quantum efficiency in …

JH Lee, HY Lin, CH Chen, YT Lee… - … Applied Materials & …, 2021 - ACS Publications
A novel bis-4Ph-substituted 9, 10-dipehnylanthracene deep blue [1931 CIE (0.15, 0.08)]
fluorescent compound, AnB4Ph, has been synthesized and characterized for organic light …

Vapor deposition of a nonmesogen prepares highly structured organic glasses

C Bishop, JL Thelen, E Gann, MF Toney, L Yu… - Proceedings of the …, 2019 - pnas.org
We show that glasses with aligned smectic liquid crystal-like order can be produced by
physical vapor deposition of a molecule without any equilibrium liquid crystal phases …

Synergistic effect of polyvinyl alcohol and copovidone in itraconazole amorphous solid dispersions

K Wlodarski, F Zhang, T Liu, W Sawicki… - Pharmaceutical …, 2018 - Springer
Purpose The first objective is to evaluate the feasibility of melt-extruding polyvinyl alcohol-
based amorphous solid dispersions for oral drug delivery. The second objective is to …