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Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …
carbon neutral through an alternative electrical approach to the energy-intensive …
Electrochemical Approaches for CO2 Conversion to Chemicals: A Journey toward Practical Applications
Conspectus Carbon capture, utilization, and sequestration play an essential role to address
CO2 emissions. Among all carbon utilization technologies, CO2 electroreduction has gained …
CO2 emissions. Among all carbon utilization technologies, CO2 electroreduction has gained …
Atomic-scale surface restructuring of copper electrodes under CO2 electroreduction conditions
R Amirbeigiarab, J Tian, A Herzog, C Qiu… - Nature Catalysis, 2023 - nature.com
Potentiodynamic methods that induce structural changes in Cu catalysts for the
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …
Accelerating electrochemical CO2 reduction to multi-carbon products via asymmetric intermediate binding at confined nanointerfaces
Abstract Electrochemical CO2 reduction (CO2R) to ethylene and ethanol enables the long-
term storage of renewable electricity in valuable multi-carbon (C2+) chemicals. However …
term storage of renewable electricity in valuable multi-carbon (C2+) chemicals. However …
Tunable CO2 electroreduction to ethanol and ethylene with controllable interfacial wettability
The mechanism of how interfacial wettability impacts the CO2 electroreduction pathways to
ethylene and ethanol remains unclear. This paper describes the design and realization of …
ethylene and ethanol remains unclear. This paper describes the design and realization of …
High carbon utilization in CO2 reduction to multi-carbon products in acidic media
Renewable electricity-powered CO2 reduction to multi-carbon (C2+) products offers a
promising route to realization of low-carbon-footprint fuels and chemicals. However, a major …
promising route to realization of low-carbon-footprint fuels and chemicals. However, a major …
Coverage-driven selectivity switch from ethylene to acetate in high-rate CO2/CO electrolysis
Tuning catalyst microenvironments by electrolytes and organic modifications is effective in
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …
improving CO2 electrolysis performance. An alternative way is to use mixed CO/CO2 feeds …
Solution-based Cu+ transient species mediate the reconstruction of copper electrocatalysts for CO2 reduction
J Vavra, GPL Ramona, F Dattila, A Kormányos… - Nature Catalysis, 2024 - nature.com
Understanding metal surface reconstruction is of the utmost importance in electrocatalysis,
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
Insight into structural evolution, active sites, and stability of heterogeneous electrocatalysts
Studying structure–activity correlations of electrocatalysts is essential for improving the
conversion of electrical to chemical energy. Recently, increasing evidence obtained by …
conversion of electrical to chemical energy. Recently, increasing evidence obtained by …
Spin states of metal centers in electrocatalysis
Understanding the electronic structure of active sites is crucial in efficient catalyst design.
The spin state, spin configurations of d-electrons, has been frequently discussed recently …
The spin state, spin configurations of d-electrons, has been frequently discussed recently …