Substitution of alcohols by N-nucleophiles via transition metal-catalyzed dehydrogenation

Q Yang, Q Wang, Z Yu - Chemical Society Reviews, 2015 - pubs.rsc.org
Transition metal-catalyzed substitution of alcohols by N-nucleophiles (or N-alkylation of
amines and related compounds with alcohols) avoids the use of alkylating agents by means …

Acceptorless dehydrogenative coupling reactions with alcohols over heterogeneous catalysts

SMAH Siddiki, T Toyao, K Shimizu - Green Chemistry, 2018 - pubs.rsc.org
Heterogeneous catalysis for the one-pot synthesis of added-value chemicals is a growing
area in green chemistry. Among various types of organic transformations that are accessible …

Direct synthesis of benzimidazoles by dehydrogenative coupling of aromatic diamines and alcohols catalyzed by cobalt

P Daw, Y Ben-David, D Milstein - ACS Catalysis, 2017 - ACS Publications
Herein, we present the base-metal-catalyzed dehydrogenative coupling of primary alcohols
and aromatic diamines to selectively form functionalized 2-substituted benzimidazoles …

Synthesis of pyrazines and quinoxalines via acceptorless dehydrogenative coupling routes catalyzed by manganese pincer complexes

P Daw, A Kumar, NA Espinosa-Jalapa… - ACS …, 2018 - ACS Publications
Base-metal catalyzed dehydrogenative self-coupling of 2-amino alcohols to selectively form
functionalized 2, 5-substituted pyrazine derivatives is presented. Also, 2-substituted …

N-Alkylation of Amines by C1–C10 Aliphatic Alcohols Using A Well-Defined Ru(II)-Catalyst. A Metal–Ligand Cooperative Approach

AK Guin, S Pal, S Chakraborty… - The Journal of …, 2023 - ACS Publications
A Ru (II)-catalyzed efficient and selective N-alkylation of amines by C1–C10 aliphatic
alcohols is reported. The catalyst [Ru (L1a)(PPh3) Cl2](1a) bearing a tridentate redox-active …

[HTML][HTML] Synthesis of ruthenium complexes and their catalytic applications: A review

J Hafeez, M Bilal, N Rasool, U Hafeez… - Arabian Journal of …, 2022 - Elsevier
Ruthenium complexes are an important class that has multiple catalytic and biological
applications. Ruthenium has a remarkably broad and diversified chemical spectrum. In the …

Borrowing Hydrogen and Acceptorless Dehydrogenative Coupling in the Multicomponent Synthesis of N‐Heterocycles: A Comparison between Base and Noble Metal …

N Hofmann, KC Hultzsch - European Journal of Organic …, 2021 - Wiley Online Library
Acceptorless dehydrogenative coupling reactions (ADC) and hydrogen transfer strategies
(HT) provide a powerful tool in the multicomponent formation of N‐heterocycles. A broad …

Zn(II)-Catalyzed Selective N-Alkylation of Amines with Alcohols Using Redox Noninnocent Azo-Aromatic Ligand as Electron and Hydrogen Reservoir

S Chakraborty, R Mondal, S Pal, AK Guin… - The Journal of …, 2022 - ACS Publications
We report a sustainable and eco-friendly approach for selective N-alkylation of various
amines by alcohols, catalyzed by a well-defined Zn (II)-catalyst, Zn (La) Cl2 (1a), bearing a …

Recent advances in the synthesis of benzimidazole derivatives from the oxidative coupling of primary amines

M Largeron, KMH Nguyen - Synthesis, 2018 - thieme-connect.com
Benzimidazole belongs to the top five most commonly used five-membered aromatic
nitrogen heterocycles among US FDA approved pharmaceuticals. Over the last few years, a …

Nickel(II)–NΛNΛO Pincer Type Complex-Catalyzed N-alkylation of Amines with Alcohols via the Hydrogen Autotransfer Reaction

G Balamurugan, R Ramesh… - The Journal of Organic …, 2020 - ACS Publications
A highly sustainable catalytic protocol for the coupling of alcohols and amines for selective
monoalkylated amines using Ni (II)–NΛNΛO pincer type complexes through the borrowing …