Atom probe tomography

B Gault, A Chiaramonti, O Cojocaru-Mirédin… - Nature Reviews …, 2021 - nature.com
Atom probe tomography (APT) provides three-dimensional compositional map** with sub-
nanometre resolution. The sensitivity of APT is in the range of parts per million for all …

A comparative review of the aqueous corrosion of glasses, crystalline ceramics, and metals

GS Frankel, JD Vienna, J Lian, JR Scully, S Gin… - npj Materials …, 2018 - nature.com
All materials can suffer from environmental degradation; the rate and extent of degradation
depend on the details of the material composition and structure as well as the environment …

Challenges with vitrification of Hanford High-Level Waste (HLW) to borosilicate glass–An overview

A Goel, JS McCloy, R Pokorny, AA Kruger - Journal of Non-Crystalline …, 2019 - Elsevier
Abstract The Hanford site in Washington State houses~ 56 million gallons of radioactive
wastes stored in 177 underground tanks. The waste must be immobilized and permanently …

Nanometre-scale evidence for interfacial dissolution–reprecipitation control of silicate glass corrosion

R Hellmann, S Cotte, E Cadel, S Malladi, LS Karlsson… - Nature materials, 2015 - nature.com
Silicate glasses are durable solids, and yet they are chemically unstable in contact with
aqueous fluids—this has important implications for numerous industrial applications related …

Origin and consequences of silicate glass passivation by surface layers

S Gin, P Jollivet, M Fournier, F Angeli, P Frugier… - Nature …, 2015 - nature.com
Silicate glasses are durable materials, but are they sufficiently durable to confine highly
radioactive wastes for hundreds of thousands years? Addressing this question requires a …

Radionuclides containment in nuclear glasses: an overview

S Gin, P Jollivet, M Tribet, S Peuget, S Schuller - Radiochimica Acta, 2017 - degruyter.com
Radioactive waste vitrification has been carried out industrially in several countries for
nearly 40 years. Research into the formulation and long term behavior of high and …

Atom probe tomography: Development and application to the geosciences

SM Reddy, DW Saxey, WDA Rickard… - Geostandards and …, 2020 - Wiley Online Library
Atom probe tomography (APT) is an analytical technique that provides quantitative three‐
dimensional elemental and isotopic analyses at sub‐nanometre resolution across the whole …

Current understanding and remaining challenges in modeling long‐term degradation of borosilicate nuclear waste glasses

JD Vienna, JV Ryan, S Gin… - International Journal of …, 2013 - Wiley Online Library
Chemical durability is not a single material property that can be uniquely measured. Instead,
it is the response to a host of coupled material and environmental processes whose rates …

The fate of silicon during glass corrosion under alkaline conditions: a mechanistic and kinetic study with the International Simple Glass

S Gin, P Jollivet, M Fournier, C Berthon, Z Wang… - … et Cosmochimica Acta, 2015 - Elsevier
Abstract International Simple Glass–a six oxide borosilicate glass selected by the
international nuclear glass community to improve the understanding of glass corrosion …

Behavior of molecules and molecular ions near a field emitter

B Gault, DW Saxey, MW Ashton, SB Sinnott… - New Journal of …, 2016 - iopscience.iop.org
The cold emission of particles from surfaces under intense electric fields is a process which
underpins a variety of applications including atom probe tomography (APT), an analytical …