Attosecond science based on high harmonic generation from gases and solids

J Li, J Lu, A Chew, S Han, J Li, Y Wu, H Wang… - Nature …, 2020 - nature.com
Recent progress in high power ultrafast short-wave and mid-wave infrared lasers has
enabled gas-phase high harmonic generation (HHG) in the water window and beyond, as …

Attosecond coherent electron motion in Auger-Meitner decay

S Li, T Driver, P Rosenberger, EG Champenois, J Duris… - Science, 2022 - science.org
In quantum systems, coherent superpositions of electronic states evolve on ultrafast time
scales (few femtoseconds to attoseconds; 1 attosecond= 0.001 femtoseconds= 10− 18 …

Attochemistry: Is controlling electrons the future of photochemistry?

ICD Merritt, D Jacquemin, M Vacher - The Journal of Physical …, 2021 - ACS Publications
Controlling matter with light has always been a great challenge, leading to the ever-
expanding field of photochemistry. In addition, since the first generation of light pulses of …

Condensed Matter Systems Exposed to Radiation: Multiscale Theory, Simulations, and Experiment

AV Solov'yov, AV Verkhovtsev, NJ Mason… - Chemical …, 2024 - ACS Publications
This roadmap reviews the new, highly interdisciplinary research field studying the behavior
of condensed matter systems exposed to radiation. The Review highlights several recent …

Long-lived electronic coherences in molecules

B Kaufman, P Marquetand, T Rozgonyi, T Weinacht - Physical Review Letters, 2023 - APS
We demonstrate long-lived electronic coherences in molecules using a combination of
measurements with shaped octave spanning ultrafast laser pulses and calculations of the …

Correlation-driven transient hole dynamics resolved in space and time in the isopropanol molecule

T Barillot, O Alexander, B Cooper, T Driver, D Garratt… - Physical Review X, 2021 - APS
The possibility of suddenly ionized molecules undergoing extremely fast electron hole (or
hole) dynamics prior to significant structural change was first recognized more than 20 years …

Manipulating attosecond charge migration in molecules by optical cavities

Y Gu, B Gu, S Sun, H Yong, VY Chernyak… - Journal of the …, 2023 - ACS Publications
The ultrafast electronic charge dynamics in molecules upon photoionization while the
nuclear motions are frozen is known as charge migration. In a theoretical study of the …

Quantum interference paves the way for long-lived electronic coherences

D Dey, AI Kuleff, GA Worth - Physical Review Letters, 2022 - APS
The creation and dynamical fate of a coherent superposition of electronic states generated
in a polyatomic molecule by broadband ionization with extreme ultraviolet pulses is studied …

Ultrafast dynamics of correlation bands following XUV molecular photoionization

M Hervé, V Despré, P Castellanos Nash, V Loriot… - Nature Physics, 2021 - nature.com
Modern ultrashort X-ray/XUV (extreme ultraviolet) sources provide unique opportunities to
investigate the primary reactions of matter upon energetic excitation. Understanding these …

Decoherence and revival in attosecond charge migration driven by non-adiabatic dynamics

DT Matselyukh, V Despré, NV Golubev, AI Kuleff… - Nature physics, 2022 - nature.com
Attosecond charge migration is a periodic evolution of the charge density at specific sites of
a molecule on a timescale defined by the energy intervals between the electronic states …