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Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …
carbon neutral through an alternative electrical approach to the energy-intensive …
Surface engineering for stable electrocatalysis
VH Do, JM Lee - Chemical Society Reviews, 2024 - pubs.rsc.org
In recent decades, significant progress has been achieved in rational developments of
electrocatalysts through constructing novel atomistic structures and modulating catalytic …
electrocatalysts through constructing novel atomistic structures and modulating catalytic …
Atomic-scale surface restructuring of copper electrodes under CO2 electroreduction conditions
R Amirbeigiarab, J Tian, A Herzog, C Qiu… - Nature Catalysis, 2023 - nature.com
Potentiodynamic methods that induce structural changes in Cu catalysts for the
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …
electrochemical reduction of CO2 (CO2RR) have been identified as a promising strategy for …
In Situ Infrared Spectroscopic Evidence of Enhanced Electrochemical CO2 Reduction and C–C Coupling on Oxide-Derived Copper
The reaction mechanism of CO2 electroreduction on oxide-derived copper has not yet been
unraveled even though high C2+ Faradaic efficiencies are commonly observed on these …
unraveled even though high C2+ Faradaic efficiencies are commonly observed on these …
Cascade electrocatalysis via AgCu single-atom alloy and Ag nanoparticles in CO2 electroreduction toward multicarbon products
C Du, JP Mills, AG Yohannes, W Wei, L Wang… - Nature …, 2023 - nature.com
Electrocatalytic CO2 reduction into value-added multicarbon products offers a means to
close the anthropogenic carbon cycle using renewable electricity. However, the …
close the anthropogenic carbon cycle using renewable electricity. However, the …
Solution-based Cu+ transient species mediate the reconstruction of copper electrocatalysts for CO2 reduction
J Vavra, GPL Ramona, F Dattila, A Kormányos… - Nature Catalysis, 2024 - nature.com
Understanding metal surface reconstruction is of the utmost importance in electrocatalysis,
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
Experimental evidence of distinct sites for CO2-to-CO and CO conversion on Cu in the electrochemical CO2 reduction reaction
The electrochemical CO2 reduction reaction on Cu is widely believed to occur via two
consecutive and orthogonal reaction steps, that is, CO2-to-CO and CO-to-C2+, on the same …
consecutive and orthogonal reaction steps, that is, CO2-to-CO and CO-to-C2+, on the same …
In situ X-ray spectroscopies beyond conventional X-ray absorption spectroscopy on deciphering dynamic configuration of electrocatalysts
Realizing viable electrocatalytic processes for energy conversion/storage strongly relies on
an atomic-level understanding of dynamic configurations on catalyst-electrolyte interface. X …
an atomic-level understanding of dynamic configurations on catalyst-electrolyte interface. X …
Electrochemical CO2 reduction (CO2RR) to multi-carbon products over copper-based catalysts
Copper has been recognized as the only heterogeneous catalyst leading to the formation of
various products of hydrocarbons and oxygenates, such as ethanol and ethylene, from the …
various products of hydrocarbons and oxygenates, such as ethanol and ethylene, from the …
Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction
J Wang, HY Tan, MY Qi, JY Li, ZR Tang… - Chemical Society …, 2023 - pubs.rsc.org
The ubiquity of solid–liquid interfaces in nature and the significant role of their atomic-scale
structure in determining interfacial properties have led to intensive research. Particularly in …
structure in determining interfacial properties have led to intensive research. Particularly in …