Measuring molecular magnets for quantum technologies

E Moreno-Pineda, W Wernsdorfer - Nature Reviews Physics, 2021 - nature.com
Single-molecule magnets (SMMs) have been proposed for applications in high-density
storage, quantum simulation, quantum computing and spintronics applications. Bulk …

Light–matter interaction at atomic scales

R Gutzler, M Garg, CR Ast, K Kuhnke, K Kern - Nature Reviews Physics, 2021 - nature.com
Light–matter interaction drives many systems, such as optoelectronic devices like light-
emitting diodes and solar cells, biological structures like photosystem II and potential future …

The second quantum revolution: role and challenges of molecular chemistry

M Atzori, R Sessoli - Journal of the American Chemical Society, 2019 - ACS Publications
Implementation of modern Quantum Technologies might benefit from the remarkable
quantum properties shown by molecular spin systems. In this Perspective, we highlight the …

Electron spin resonance of single iron phthalocyanine molecules and role of their non-localized spins in magnetic interactions

X Zhang, C Wolf, Y Wang, H Aubin, T Bilgeri… - Nature Chemistry, 2022 - nature.com
Electron spin resonance (ESR) spectroscopy is a crucial tool, through spin labelling, in
investigations of the chemical structure of materials and of the electronic structure of …

A quantum sensor for atomic-scale electric and magnetic fields

T Esat, D Borodin, J Oh, AJ Heinrich, FS Tautz… - Nature …, 2024 - nature.com
The detection of faint magnetic fields from single-electron and nuclear spins at the atomic
scale is a long-standing challenge in physics. While current mobile quantum sensors …

Coherent spin manipulation of individual atoms on a surface

K Yang, W Paul, SH Phark, P Willke, Y Bae, T Choi… - Science, 2019 - science.org
Achieving time-domain control of quantum states with atomic-scale spatial resolution in
nanostructures is a long-term goal in quantum nanoscience and spintronics. Here, we …

Construction of topological quantum magnets from atomic spins on surfaces

H Wang, P Fan, J Chen, L Jiang, HJ Gao… - Nature …, 2024 - nature.com
Artificial quantum systems have emerged as platforms to realize topological matter in a well-
controlled manner. So far, experiments have mostly explored non-interacting topological …

Creating designer quantum states of matter atom-by-atom

AA Khajetoorians, D Wegner, AF Otte, I Swart - Nature Reviews Physics, 2019 - nature.com
Advances in high-resolution and spin-resolved scanning tunnelling microscopy, as well as
atomic-scale manipulation, have enabled the bottom-up, atom-by-atom creation and …

Coherent spin control of single molecules on a surface

P Willke, T Bilgeri, X Zhang, Y Wang, C Wolf, H Aubin… - ACS …, 2021 - ACS Publications
Control of single electron spins constitutes one of the most promising platforms for
spintronics, quantum sensing, and quantum information processing. Utilizing single …

Free coherent evolution of a coupled atomic spin system initialized by electron scattering

LM Veldman, L Farinacci, R Rejali, R Broekhoven… - Science, 2021 - science.org
Full insight into the dynamics of a coupled quantum system depends on the ability to follow
the effect of a local excitation in real-time. Here, we trace the free coherent evolution of a pair …