Recent progress in the phase-transition mechanism and modulation of vanadium dioxide materials
Metal-to-insulator transition (MIT) behaviors accompanied by a rapid reversible phase
transition in vanadium dioxide (VO2) have gained substantial attention for investigations into …
transition in vanadium dioxide (VO2) have gained substantial attention for investigations into …
Ultrafast dynamics during the photoinduced phase transition in VO2
The phase transition of VO 2 from a monoclinic insulator to a rutile metal, which occurs
thermally at TC= 340 K, can also be driven by strong photoexcitation. The ultrafast dynamics …
thermally at TC= 340 K, can also be driven by strong photoexcitation. The ultrafast dynamics …
A photoinduced metal-like phase of monoclinic VO2 revealed by ultrafast electron diffraction
The complex interplay among several active degrees of freedom (charge, lattice, orbital, and
spin) is thought to determine the electronic properties of many oxides. We report on …
spin) is thought to determine the electronic properties of many oxides. We report on …
Ultrafast X-ray imaging of the light-induced phase transition in VO2
Using light to control transient phases in quantum materials is an emerging route to
engineer new properties and functionality, with both thermal and non-thermal phases …
engineer new properties and functionality, with both thermal and non-thermal phases …
Tracking the insulator-to-metal phase transition in VO2 with few-femtosecond extreme UV transient absorption spectroscopy
Coulomb correlations can manifest in exotic properties in solids, but how these properties
can be accessed and ultimately manipulated in real time is not well understood. The …
can be accessed and ultimately manipulated in real time is not well understood. The …
Instantaneous Band Gap Collapse in Photoexcited Monoclinic due to Photocarrier Do**
Using femtosecond time-resolved photoelectron spectroscopy we demonstrate that
photoexcitation transforms monoclinic VO 2 quasi-instantaneously into a metal. Thereby, we …
photoexcitation transforms monoclinic VO 2 quasi-instantaneously into a metal. Thereby, we …
Inhomogeneity of the ultrafast insulator-to-metal transition dynamics of VO2
The insulator-metal transition (IMT) of vanadium dioxide (VO2) has remained a long-
standing challenge in correlated electron physics since its discovery five decades ago. Most …
standing challenge in correlated electron physics since its discovery five decades ago. Most …
Tracking ultrafast solid-state dynamics using high harmonic spectroscopy
We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy
method for tracking photoinduced dynamics in strongly correlated materials through a …
method for tracking photoinduced dynamics in strongly correlated materials through a …
How optical excitation controls the structure and properties of vanadium dioxide
We combine ultrafast electron diffraction and time-resolved terahertz spectroscopy
measurements to link structure and electronic transport properties during the photoinduced …
measurements to link structure and electronic transport properties during the photoinduced …
Vanadium dioxide for dynamically tunable photonics
As the quest for active photonic devices continues, materials with exotic and exploitable
properties have become paramount to enable new advancements. In recent years, phase …
properties have become paramount to enable new advancements. In recent years, phase …