The Structure of Active Centers and the Ethylene Polymerization Mechanism on the Cr/SiO2 Catalyst:  A Frontier for the Characterization Methods

E Groppo, C Lamberti, S Bordiga, G Spoto… - Chemical …, 2005 - ACS Publications
The discovery of olefin polymerization catalysts in the early 1950s by Ziegler and Natta
represents a milestone in industrial catalysis. This discovery was of outstanding relevance …

Interplay of electronic, environmental, and vibrational effects in determining the hyperfine coupling constants of organic free radicals

R Improta, V Barone - Chemical reviews, 2004 - ACS Publications
Organic free radicals are ubiquitous in chemical and biological systems. They are involved
in a huge number of fundamental processes going from simple organic reactions1-3 through …

Toward the prediction of magnetic coupling in molecular systems: hydroxo-and alkoxo-bridged Cu (II) binuclear complexes

E Ruiz, P Alemany, S Alvarez… - Journal of the American …, 1997 - ACS Publications
Magnetic coupling constants (2 J) of hydroxo-and alkoxo-bridged copper binuclear
compounds have been evaluated to determine the accuracy of different density functional …

A computational analysis of substituent effects on the O− H bond dissociation energy in phenols: polar versus radical effects

T Brinck, M Haeberlein, M Jonsson - Journal of the American …, 1997 - ACS Publications
O− H bond dissociation energies (BDEs) of phenol, p-aminophenol, and p-nitrophenol have
been computed using ab initio and density functional theory (DFT) methods. The MP2 and …

An accurate density functional method for the study of magnetic properties: the PBE0 model

C Adamo, M Cossi, V Barone - Journal of Molecular Structure: THEOCHEM, 1999 - Elsevier
We analyze the quality of the magnetic properties computed by a parameter free density
functional model (PBE0) obtained by combining the PBE generalized gradient functional …

Mechanism of the reaction

IS Ignatyev, Y **e, WD Allen… - The Journal of chemical …, 1997 - pubs.aip.org
The geometries, energies, and vibrational frequencies of the reactants, transition states,
intermediates, and products of the reaction of ethyl radical with the oxygen molecule have …

Water concentration profiles in membranes measured by ESEEM of spin-labeled lipids

DA Erilov, R Bartucci, R Guzzi, AA Shubin… - The Journal of …, 2005 - ACS Publications
Electron spin− echo envelope modulation (ESEEM) spectroscopy of phospholipids spin-
labeled systematically down the sn-2 chain was used to detect the penetration of water …

Theoretical investigation on the role of the central carbon atom and close protein environment on the nitrogen reduction in Mo nitrogenase

L Rao, X Xu, C Adamo - ACS Catalysis, 2016 - ACS Publications
A theoretical study elucidating the mechanism of N2 reduction in Mo nitrogenase was
carried out using a QM/QM′ approach based on density functional theory/semiempirical …

Accurate calculations of bond dissociation enthalpies with density functional methods

XQ Yao, XJ Hou, H Jiao, HW **ang… - The Journal of Physical …, 2003 - ACS Publications
The homolytic dissociation enthalpies of various bonds (C− H, N− H, O− H, S− H, X− H, C−
C, C− N, C− O, C− S, and C− halogen) have been computed by using five density functional …

Nuclear magnetic resonance shifts in paramagnetic metalloporphyrins and metalloproteins

J Mao, Y Zhang, E Oldfield - Journal of the American Chemical …, 2002 - ACS Publications
We report the first detailed investigation of the 1H, 13C, 15N, and 19F nuclear magnetic
resonance (NMR) spectroscopic shifts in paramagnetic metalloprotein and metalloporphyrin …