Generalized spin in the variance-based wave function optimization method within the doubly occupied configuration interaction framework

DR Alcoba, L Lain, A Torre, TR Ayala… - The Journal of …, 2024 - ACS Publications
In this work, we implement a generalized spin formulation of the doubly occupied
configuration interaction methodology using the energy variance of the N-electron …

Quantum Information Patterns Between Atoms in a Molecule

D Van Hende, R Van der Stichelen… - … A European Journal, 2024 - Wiley Online Library
Quantum information theory provides a powerful toolbox of descriptors that characterize
many‐electron systems based on quantum information patterns between open quantum …

Capturing correlation in the spin frustrated H3-ring using the generator coordinate method and spin-constrained generalised Hartree-Fock states

X De Vriendt, J De Vos, S De Baerdemacker… - Molecular …, 2023 - Taylor & Francis
In spin frustrated H 3-rings, variationally minimal single Slater determinant descriptions
break S^ 2 and S^ z symmetries in an effort to simultaneously minimise the interactions …

Spin-constrained Hartree–Fock and the generator coordinate method for the 2-site Hubbard model

S De Baerdemacker, A Ayati, HGA Burton… - Advances in Quantum …, 2023 - Elsevier
We present a mathematical analysis of the spin-constrained Hartree–Fock solutions (CHF)
of the 2-site Hubbard model. The analysis sheds light on the spin-symmetry breaking …