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Electrochemical CO2 reduction (CO2RR) to multi-carbon products over copper-based catalysts
Copper has been recognized as the only heterogeneous catalyst leading to the formation of
various products of hydrocarbons and oxygenates, such as ethanol and ethylene, from the …
various products of hydrocarbons and oxygenates, such as ethanol and ethylene, from the …
Construction of C–N bonds from small-molecule precursors through heterogeneous electrocatalysis
Energy-intensive thermochemical processes within chemical manufacturing are a major
contributor to global CO2 emissions. With the increasing push for sustainability, the scientific …
contributor to global CO2 emissions. With the increasing push for sustainability, the scientific …
Operando studies reveal active Cu nanograins for CO2 electroreduction
Carbon dioxide electroreduction facilitates the sustainable synthesis of fuels and chemicals.
Although Cu enables CO2-to-multicarbon product (C2+) conversion, the nature of the active …
Although Cu enables CO2-to-multicarbon product (C2+) conversion, the nature of the active …
Solution-based Cu+ transient species mediate the reconstruction of copper electrocatalysts for CO2 reduction
Understanding metal surface reconstruction is of the utmost importance in electrocatalysis,
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
as this phenomenon directly affects the nature of available active sites. However, its dynamic …
Well-defined diatomic catalysis for photosynthesis of C2H4 from CO2
Z **e, S Xu, L Li, S Gong, X Wu, D Xu, B Mao… - Nature …, 2024 - nature.com
Owing to the specific electronic-redistribution and spatial proximity, diatomic catalysts
(DACs) have been identified as principal interest for efficient photoconversion of CO2 into …
(DACs) have been identified as principal interest for efficient photoconversion of CO2 into …
Operando scanning electrochemical probe microscopy during electrocatalysis
Scanning electrochemical probe microscopy (SEPM) techniques can disclose the local
electrochemical reactivity of interfaces in single-entity and sub-entity studies. Operando …
electrochemical reactivity of interfaces in single-entity and sub-entity studies. Operando …
Confined growth of silver–copper Janus nanostructures with {100} facets for highly selective tandem electrocatalytic carbon dioxide reduction
Electrocatalytic carbon dioxide reduction reaction (CO2RR) holds significant potential to
promote carbon neutrality. However, the selectivity toward multicarbon products in CO2RR …
promote carbon neutrality. However, the selectivity toward multicarbon products in CO2RR …
Linking the Dynamic Chemical State of Catalysts with the Product Profile of Electrocatalytic CO2 Reduction
The promoted activity and enhanced selectivity of electrocatalysts is commonly ascribed to
specific structural features such as surface facets, morphology, and atomic defects …
specific structural features such as surface facets, morphology, and atomic defects …
Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
The electrocatalytic reduction of carbon dioxide is a promising approach for storing (excess)
renewable electricity as chemical energy in fuels. Here, we review recent advances and …
renewable electricity as chemical energy in fuels. Here, we review recent advances and …
The role of in situ generated morphological motifs and Cu(i) species in C2+ product selectivity during CO2 pulsed electroreduction
The efficient electrochemical conversion of CO2 provides a route to fuels and feedstocks.
Copper catalysts are well-known to be selective to multicarbon products, although the role …
Copper catalysts are well-known to be selective to multicarbon products, although the role …