From femtoseconds to hours—measuring dynamics over 18 orders of magnitude with coherent x-rays

F Lehmkühler, W Roseker, G Grübel - Applied Sciences, 2021 - mdpi.com
X-ray photon correlation spectroscopy (XPCS) enables the study of sample dynamics
between micrometer and atomic length scales. As a coherent scattering technique, it …

Cascaded hard X-ray self-seeded free-electron laser at megahertz repetition rate

S Liu, C Grech, M Guetg, S Karabekyan… - Nature …, 2023 - nature.com
High-resolution X-ray spectroscopy in the sub-nanosecond to femtosecond time range
requires ultrashort X-ray pulses and a spectral X-ray flux considerably larger than that …

Exploring non-equilibrium processes and spatio-temporal scaling laws in heated egg yolk using coherent X-rays

ND Anthuparambil, A Girelli, S Timmermann… - Nature …, 2023 - nature.com
The soft-grainy microstructure of cooked egg yolk is the result of a series of out-of-
equilibrium processes of its protein-lipid contents; however, it is unclear how egg yolk …

Resolving molecular diffusion and aggregation of antibody proteins with megahertz X-ray free-electron laser pulses

M Reiser, A Girelli, A Ragulskaya, S Das… - Nature …, 2022 - nature.com
X-ray free-electron lasers (XFELs) with megahertz repetition rate can provide novel insights
into structural dynamics of biological macromolecule solutions. However, very high dose …

AI-NERD: Elucidation of relaxation dynamics beyond equilibrium through AI-informed X-ray photon correlation spectroscopy

JP Horwath, XM Lin, H He, Q Zhang… - Nature …, 2024 - nature.com
Understanding and interpreting dynamics of functional materials in situ is a grand challenge
in physics and materials science due to the difficulty of experimentally probing materials at …

Refractive guide switching a regenerative amplifier free-electron laser for high peak and average power hard x rays

G Marcus, A Halavanau, Z Huang, J Krzywinski… - Physical Review Letters, 2020 - APS
We present an x-ray regenerative amplifier free-electron laser design capable of producing
fully coherent hard x-ray pulses across a broad tuning range at a high steady state repetition …

Intermittent Defect Fluctuations in Oxide Heterostructures

Q Zhang, G Wan, V Starchenko, G Hu… - Advanced …, 2023 - Wiley Online Library
The heterogeneous nature, local presence, and dynamic evolution of defects typically
govern the ionic and electronic properties of a wide variety of functional materials. While the …

Real-time swelling-collapse kinetics of nanogels driven by XFEL pulses

F Dallari, I Lokteva, J Möller, W Roseker, C Goy… - Science …, 2024 - science.org
Stimuli-responsive polymers are an important class of materials with many applications in
nanotechnology and drug delivery. The most prominent one is poly-N-isopropylacrylamide …

Operational experience with adaptive gain integrating pixel detectors at European XFEL

J Sztuk-Dambietz, V Rovensky, A Klujev, T Laurus… - Frontiers in …, 2024 - frontiersin.org
The European X-ray Free Electron Laser (European XFEL) is a cutting-edge user facility that
generates per second up to 27,000 ultra-short, spatially coherent X-ray pulses within an …

[PDF][PDF] Microsecond hydrodynamic interactions in dense colloidal dispersions probed at the European XFEL

F Dallari, A Jain, M Sikorski, J Möller, R Bean… - IUCrJ, 2021 - journals.iucr.org
Many soft-matter systems are composed of macromolecules or nanoparticles suspended in
water. The characteristic times at intrinsic length scales of a few nanometres fall therefore in …