Multiscale CO2 Electrocatalysis to C2+ Products: Reaction Mechanisms, Catalyst Design, and Device Fabrication

T Yan, X Chen, L Kumari, J Lin, M Li, Q Fan… - Chemical …, 2023 - ACS Publications
Electrosynthesis of value-added chemicals, directly from CO2, could foster achievement of
carbon neutral through an alternative electrical approach to the energy-intensive …

Spatially and temporally understanding dynamic solid–electrolyte interfaces in carbon dioxide electroreduction

J Wang, HY Tan, MY Qi, JY Li, ZR Tang… - Chemical Society …, 2023 - pubs.rsc.org
The ubiquity of solid–liquid interfaces in nature and the significant role of their atomic-scale
structure in determining interfacial properties have led to intensive research. Particularly in …

Absence of CO2 electroreduction on copper, gold and silver electrodes without metal cations in solution

MCO Monteiro, F Dattila, B Hagedoorn… - Nature Catalysis, 2021 - nature.com
The electrocatalytic reduction of carbon dioxide is widely studied for the sustainable
production of fuels and chemicals. Metal ions in the electrolyte influence the reaction …

Localized Alkaline Environment via In Situ Electrostatic Confinement for Enhanced CO2-to-Ethylene Conversion in Neutral Medium

Z Wang, Y Li, X Zhao, S Chen, Q Nian… - Journal of the …, 2023 - ACS Publications
Electrocatalytic CO2 reduction reaction (CO2RR) is one of the most promising routes to
facilitate carbon neutrality. An alkaline electrolyte is typically needed to promote the …

Industrial-Current-Density CO2-to-C2+ Electroreduction by Anti-swelling Anion-Exchange Ionomer-Modified Oxide-Derived Cu Nanosheets

Y Zhao, X Zu, R Chen, X Li, Y Jiang… - Journal of the …, 2022 - ACS Publications
CO2 electroreduction to high-energy-density C2+ products is highly attractive, whereas the
C2+ selectivity under industrial current densities is still unsatisfying. Here, an anti-swelling …

Activating dynamic atomic-configuration for single-site electrocatalyst in electrochemical CO2 reduction

CS Hsu, J Wang, YC Chu, JH Chen, CY Chien… - Nature …, 2023 - nature.com
One challenge for realizing high-efficiency electrocatalysts for CO2 electroreduction is
lacking in comprehensive understanding of potential-driven chemical state and dynamic …

Asymmetric Low-Frequency Pulsed Strategy Enables Ultralong CO2 Reduction Stability and Controllable Product Selectivity

XD Zhang, T Liu, C Liu, DS Zheng… - Journal of the …, 2023 - ACS Publications
Copper-based catalysts are widely explored in electrochemical CO2 reduction (CO2RR)
because of their ability to convert CO2 into high-value-added multicarbon products …

Electrochemical surface-enhanced Raman spectroscopy

CL Brosseau, A Colina, JV Perales-Rondon… - Nature Reviews …, 2023 - nature.com
Electrochemical surface-enhanced Raman spectroscopy (EC-SERS) is a
spectroelectrochemical method that has been in existence since the first SERS …

Different distributions of multi-carbon products in CO2 and CO electroreduction under practical reaction conditions

JYT Kim, C Sellers, S Hao, TP Senftle, H Wang - Nature Catalysis, 2023 - nature.com
Product selectivity differences between the electroreduction of CO2 and CO under practical
current densities are a widely encountered phenomenon that is rarely emphasized or …

In-situ/operando Raman techniques for in-depth understanding on electrocatalysis

M Chen, D Liu, L Qiao, P Zhou, J Feng, KW Ng… - Chemical Engineering …, 2023 - Elsevier
Recently, the electrocatalysis has attracted increasing attention for the sustainable
development of society, which has been applied for energy harvesting/storage and pollution …