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Expanded theory of H-and J-molecular aggregates: the effects of vibronic coupling and intermolecular charge transfer
The electronic excited states of molecular aggregates and their photophysical signatures
have long fascinated spectroscopists and theoreticians alike since the advent of Frenkel …
have long fascinated spectroscopists and theoreticians alike since the advent of Frenkel …
Exciton–vibrational coupling in the dynamics and spectroscopy of Frenkel excitons in molecular aggregates
The influence of exciton–vibrational coupling on the optical and transport properties of
molecular aggregates is an old problem that gained renewed interest in recent years. On the …
molecular aggregates is an old problem that gained renewed interest in recent years. On the …
Perspectives in dye chemistry: a rational approach toward functional materials by understanding the aggregate state
The past 20 years have witnessed a renaissance of dye chemistry, moving from traditional
colorant research toward functional materials. Different from traditional colorant research …
colorant research toward functional materials. Different from traditional colorant research …
Origin of long-lived coherences in light-harvesting complexes
N Christensson, HF Kauffmann… - The Journal of …, 2012 - ACS Publications
A vibronic exciton model is applied to explain the long-lived oscillatory features in the two-
dimensional (2D) electronic spectra of the Fenna–Matthews–Olson (FMO) complex. Using …
dimensional (2D) electronic spectra of the Fenna–Matthews–Olson (FMO) complex. Using …
Quantum phase synchronization via exciton-vibrational energy dissipation sustains long-lived coherence in photosynthetic antennas
The lifetime of electronic coherences found in photosynthetic antennas is known to be too
short to match the energy transfer time, rendering the coherent energy transfer mechanism …
short to match the energy transfer time, rendering the coherent energy transfer mechanism …
Vibronic mixing enables ultrafast energy flow in light-harvesting complex II
Since the discovery of quantum beats in the two-dimensional electronic spectra of
photosynthetic pigment-protein complexes over a decade ago, the origin and mechanistic …
photosynthetic pigment-protein complexes over a decade ago, the origin and mechanistic …
Enhancement of vibronic and ground-state vibrational coherences in 2D spectra of photosynthetic complexes
A vibronic-exciton model is applied to investigate the recently proposed mechanism of
enhancement of coherent oscillations due to mixing of electronic and nuclear degrees of …
enhancement of coherent oscillations due to mixing of electronic and nuclear degrees of …
Quantum coherences reveal excited-state dynamics in biophysical systems
Ultrafast, multi-dimensional spectroscopic measurements of photosynthetic light-harvesting
complexes have revealed quantum coherences with timescales comparable to those of …
complexes have revealed quantum coherences with timescales comparable to those of …
Multi-layer multi-configuration time-dependent Hartree (ML-MCTDH) approach to the correlated exciton-vibrational dynamics in the FMO complex
The coupled quantum dynamics of excitonic and vibrational degrees of freedom is
investigated for high-dimensional models of the Fenna-Matthews-Olson complex. This …
investigated for high-dimensional models of the Fenna-Matthews-Olson complex. This …
Coherent exciton delocalization in a two-state DNA-templated dye aggregate system
Coherent exciton delocalization in dye aggregate systems gives rise to a variety of intriguing
optical phenomena, including J-and H-aggregate behavior and Davydov splitting. Systems …
optical phenomena, including J-and H-aggregate behavior and Davydov splitting. Systems …